In this effort, an assessment of bulk ultrasonic (UT) and eddy current (ECT) methods and techniques is performed for inspecting the surfaces of dry cask storage systems (DCSSs) canisters. Some DCSS canisters (especially those located in coastal environments) will be exposed to environmental conditions, which can cause atmospheric stress corrosion cracking (SCC). Information collected from the field and from laboratory studies has not been able to rule out the possibility of atmospheric SCC in DCSS canisters, although no occurrences of atmospheric SCC in DCSS canisters have been detected. UT and ECT methods and techniques are already used to inspect nuclear power plant components and this experience, along with their relative maturity, makes these methods and techniques likely frontrunners for near-term application to examination of dry storage canister surfaces. In this report, the results of several performance reliability studies for UT and ECT are reviewed. The detection, depth-sizing, and lengthsizing results are documented and summarized to quantitatively estimate the adequacy of UT and ECT for inspecting dry storage canister surfaces. In addition, this effort focuses on the implementation of NDE methods and techniques in the Holtec HI-STORM 100 system and the Transnuclear NUHOMS horizontal storage modules and considers environmental compatibility, accessibility constraints, and NDE sensor deployment options for these systems.v