2022
DOI: 10.26434/chemrxiv-2022-nb0fw
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Room-Temperature Reversible Chemisorption of Carbon Monoxide on Nickel(0) Complexes

Abstract: Chemisorption on organometallic-based adsorbents is crucial for the controlled separation and long-term storage of gaseous molecules. The formation of covalent bonds between the metal centers in the adsorbents and the targeted gases affects the desorption efficiency, especially when the oxidation state of the metal is low. Herein, we report a pressure-responsive nickel(0)-based system that is able to reversibly chemisorb carbon monoxide (CO) at room temperature. The use of N-heterocyclic carbene ligands with h… Show more

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