Dry
adhesives that combine strong adhesion, high transparency,
and reusability are needed to support developments in emerging fields
such as medical electrodes and the bonding of electronic optical devices.
However, achieving all of these features in a single material remains
challenging. Herein, we propose a pressure-responsive polyurethane
(PU) adhesive inspired by the octopus sucker. This adhesive not only
showcases reversible adhesion to both solid materials and biological
tissues but also exhibits robust stability and high transparency (>90%).
As the adhesive strength of the PU adhesive corresponds to the application
force, adhesion could be adjusted by the preloading force and/or pressure.
The adhesive exhibits high static adhesion (∼120 kPa) and 180°
peeling force (∼500 N/m), which is far stronger than those
of most existing artificial dry adhesives. Moreover, the adhesion
strength is effectively maintained even after 100 bonding–peeling
cycles. Because the adhesive tape relies on the combination of negative
pressure and intermolecular forces, it overcomes the underlying problems
caused by glue residue like that left by traditional glue tapes after
removal. In addition, the PU adhesive also shows wet-cleaning performance;
the contaminated tape can recover 90–95% of the lost adhesion
strength after being cleaned with water. The results show that an
adhesive with a microstructure designed to increase the contribution
of negative pressure can combine high reversible adhesion and long
fatigue life.