Electric power industry is continually adopting new techniques to improve the reliability and efficiency of the energy system and to cope with the increasing energy demand and the associated technical challenges. In recent years, the maturation of Artificial Intelligence (AI) led researchers to solve various problems in the power system by using AI techniques. Voltage Source Converter is the result of advancements in the field of power electronics and semiconductors technology, which holds a promising future for the realization of smart grid, renewable energy integration, and HVDC transmission system. Usually hit and trial method or the design engineer’s experience is used for the manual tuning of the PI controllers, which cannot yield superior performance. The process becomes more complicated when multiple grids are involved, such as in VSC-based MTDC grids. This research article use a deep learning optimization technique for the tuning of the VSC controllers, which resulted in quick settling time, better slew rate, less undershoot and low overshoot. The deep learning neural network is trained through the Particle Swarm Optimization (PSO) algorithm to produce the best possible tuned or optimally tuned parameters for the controllers. The optimal tuning of the controller will result in an overall better performance of the converter and the grid. A four-layered deep learning neural network and a three-terminal MTDC grid were designed and simulated in MATLAB/SIMULINK environment.