Nanolasers based on surface plasmon opens up new platform for advanced nanophotonics technologies. [1][2][3][4][5][6] As Raman scattering process convert pump laser into new frequencies, so development of Raman nanolaser may allows for tunable nanolasers and boost the development of innovative nanophotonics technology. The Raman conversion for conventional Raman laser is intrinsically challenging as high intensities of the pump laser are required to drive the nonlinear effect. In recent years, miniaturization of Raman silicon laser has been successfully achieved with the assistance of reverse-biased p-i-n diode at centimeter size or photonics-crystal with high-quality-factor nanocavity at micrometer size. [7][8][9] However, for applications such as high-resolution medical imagings or on-chip optical communications, 'ultimate' nanolasers with scalable, thresholdless,