We present a highly efficient picosecond diamond Raman laser synchronously-pumped by a 4.8 W mode-locked laser at 1064 nm. A ring cavity was adopted for efficient operation. With a low-Q cavity for first-Stokes 1240 nm, we have achieved 2.75 W output power at 1240 nm with 59% overall conversion efficiency. The slope efficiency tended towards 76% far above the SRS threshold, approaching the SRS quantum limit for diamond. A high-Q first-Stokes cavity was employed for second-Stokes 1485 nm generation through the combined processes of four-wave mixing and single-pass stimulated Raman scattering. Up to 1.0 W of second-stokes at 1485 nm was obtained, corresponding to 21% overall conversion efficiency. The minimum output pulse duration was compressed relative to the 15 ps pump, producing pulses as short as 9 ps for 1240 nm and 6 ps for 1485 nm respectively.

We report a synchronously-pumped femtosecond diamond Raman laser operating at 890 nm with a slope efficiency of 32%. Pumped using a mode-locked Ti:Sapphire laser at 796 nm with a pulse duration of 194 fs, the bandwidth of the Stokes output was broadened to enable subsequent pulse compression to 65 fs using a prism-pair. Modelling results provide an understanding of the physical mechanisms involved in the Raman conversion of femtosecond pulses, supporting an in-depth characterization of these ultrashort pulsed lasers.

Spectral broadening of the fundamental field in intracavity Raman lasers is investigated. The mechanism for the spectral broadening is discussed and the effect is compared in two lasers using Raman crystals with different Raman linewidths. The impact of the spectral broadening on the effective Raman gain is analyzed, and the use of etalons to limit the fundamental spectral width is explored. It was found that an improvement in output power could be obtained by using etalons to limit the fundamental spectrum to a single narrow peak. 9810-9818 (2012). 20. J. J. Zayhowski, "The effects of spatial hole burning and energy diffusion on the single-mode operation of standing-wave lasers," IEEE J. Quantum Electron.

We report a synchronously pumped femtosecond diamond Raman laser operating at 895 nm with a 33% slope efficiency. Pumped using a mode-locked Ti:sapphire laser at 800 nm with a duration of 170 fs, the bandwidth of the Stokes output is broadened and chirped to enable subsequent pulse compression to 95 fs using a prism pair. Modeling results indicate that self-phase modulation drives the broadening of the Stokes spectrum in this highly transient laser. Our results demonstrate the potential for Raman conversion to extend the wavelength coverage and pulse shorten Ti:sapphire lasers.

A Nd:YLF/KGW Raman laser has been investigated in this work. We have demonstrated CW output powers at six different wavelengths, 1147 nm (0.70 W), 1163 nm (0.95 W), 549 nm (0.65 W), 552 nm (1.90 W), 573 nm (0.60 W) and 581 nm (1.10 W), with higher peak powers achieved under quasi-CW operation. Raman conversion of the 1053 nm fundamental emission is reported for the first time, enabling two new wavelengths in crystalline Raman lasers, 549 nm and 552 nm. The weak thermal lensing associated with Nd:YLF has enabled to achieve good beam quality, M(2) ≤ 2.0, and stable operation in relatively long cavities.