The spin current pumped by a precessing ferromagnet into an adjacent normal metal has a constant polarization component parallel to the precession axis and a rotating one normal to the magnetization. The former is now routinely detected as a dc voltage induced by the inverse spin Hall effect (ISHE). Here we compute ac ISHE voltages much larger than the dc signals for various material combinations and discuss optimal conditions to observe the effect. The backflow of spin is shown to be essential to distill parameters from measured ISHE voltages for both dc and ac configurations. DOI: 10.1103/PhysRevLett.110.217602 PACS numbers: 76.50.+g, 72.25.Mk, 73.40.Àc In magnetoelectronics the electronic spin degree of freedom creates new functionalities that lead to applications in information technologies such as sensors and memories [1]. Central to much excitement in this field is the spin Hall effect (SHE) [2][3][4][5], i.e., the spin current induced normal to an applied charge current in the presence of spin-orbit interaction, as discovered optically in semiconductors [6,7] and subsequently electrically in metals [8][9][10]. Recently magnetization reversal by the SHE induced spin transfer torque has been demonstrated [11,12]. The generation of a voltage by a spin current injected into a paramagnetic metal, the inverse spin Hall effect (ISHE), can be employed to detect the spin current due to spin pumping [13][14][15] by an adjacent ferromagnet under ferromagnetic resonance (FMR) conditions [8,16]. The ISHE has also been essential for the discovery of the spin Seebeck effect [17].In recent experiments, dc voltages induced by the ISHE have been measured in many material combinations, thereby giving access to crucial parameters such as the spin Hall angle [18][19][20] and the spin mixing conductance [21], the material parameter determining, e.g., the effectiveness of interface spin-transfer torques [14]. For example, the magnitude and sign of the spin Hall angle has been determined for Permalloy ðPyÞjN bilayers for different normal metals N [18,19]. An approximate scaling relation for the spin pumping by numerous ferromagnets (F) has been discovered by comparing different FjPt bilayers as a function of excitation power [21]. However, it is far from easy to derive quantitative information from ISHE experiments [22]. As reviewed by the Cornell Collaboration [23], several experimental pitfalls should be avoided. At FMR, the dc ISHE voltage is small, scaling quadratically with the cone angle of the precessing magnetization. An important correction is caused by the back diffusion (''backflow'') of injected spins to the interface, which effectively reduces the spin current injection [14] and generates voltages normal to the interface [24,25]. This backflow has often been neglected in interpreting spin-pumping experiments, assuming that Pt, the metal of choice, can be treated like a perfect spin sink.The spin current injected by FMR into a normal metal consists of a dc component along the z axis parallel to the effective fiel...