2020
DOI: 10.1103/physrevresearch.2.033341
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Spin selection in single-frequency two-photon excitation of alkali-metal atoms

Abstract: We develop a theoretical framework for spin selection in single-frequency two-photon excitation of alkalimetal atoms as a function of polarization of the excitation light. We verify the theory by experimentally probing the 5S 1/2 → 6S 1/2 transition rate in 87 Rb in two configurations: paraxial light excitation of warm vapor and nonparaxial excitation of laser-cooled atoms. The transition rate follows a quadratic dependence on the helicity parameter linked to the excitation light's polarization. For paraxial e… Show more

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Cited by 11 publications
(8 citation statements)
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“…For 762 nm light, the output power was 1.23 mW whereas 1.3 mW was used in the model. Note that we had particularly high losses in the ONF likely due to the fact that it was 5 years old and had been used extensively for several earlier experiments [5,6,20]. After the experiment, we removed the fiber from the setup and imaged it using a scanning electron microscope; large deposits were clearly visible on it and we assume that these were Rb.…”
Section: Resultsmentioning
confidence: 99%
See 1 more Smart Citation
“…For 762 nm light, the output power was 1.23 mW whereas 1.3 mW was used in the model. Note that we had particularly high losses in the ONF likely due to the fact that it was 5 years old and had been used extensively for several earlier experiments [5,6,20]. After the experiment, we removed the fiber from the setup and imaged it using a scanning electron microscope; large deposits were clearly visible on it and we assume that these were Rb.…”
Section: Resultsmentioning
confidence: 99%
“…For Rb atoms, few such wavelengths exist, and compensation can only be achieved for pure linear or pure circular polarization of the trapping fields, and only for some upper energy levels [15]. Notably, pure polarization cannot be achieved in the evanescent field of the ONF [16][17][18][19][20].…”
Section: Introductionmentioning
confidence: 99%
“…We prepared an ensemble of trapped cold 87 Rb atoms using a standard magneto-optical trap (MOT) setup [13]. The average temperature of the atomic cloud was ∼200 μK, with a density of 10 10 atoms cm −3 .…”
Section: Methodsmentioning
confidence: 99%
“…We focus our discussion on ONFs, which provide tight confinement of light beyond the Rayleigh range and also serve as an ideal channel for light propagation. ONFs have been used to efficiently probe, manipulate and trap cold, alkali atoms [6][7][8][9][10] with recent works extending atom and ONF studies to the observation of a quadrupole transition in 87 Rb atoms [11], the demonstration of quadrature squeezing of nanofibreguided light [12], and a determination of the polarization dependency of spin selection in laser-cooled atoms [13].…”
Section: Introductionmentioning
confidence: 99%
“…This Cs transition is well known as a dipole-forbidden but a quadrupole-allowed transition. In evaluating the rate of OAM transfer involving a quadrupole transition we had to consider the relevant selection rules which involve both spin and OAM [26].…”
Section: Introductionmentioning
confidence: 99%