2021
DOI: 10.1002/advs.202103361
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State‐of‐the‐Art Advancements in Photocatalytic Hydrogenation: Reaction Mechanism and Recent Progress in Metal‐Organic Framework (MOF)‐Based Catalysts

Abstract: Photocatalytic hydrogenation provides an effective alternative way for the synthesis of industrial chemicals to meet the economic and environment expectations. Especially, over the past few years, metal-organic frameworks (MOFs), featured with tunable structure, porosity, and crystallinity, have been significantly developed as many high-performance catalysts in the field of photocatalysis. In this review, the background and development of photocatalytic hydrogenation are systemically summarized. In particular,… Show more

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Cited by 61 publications
(37 citation statements)
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“…The performance is also higher than many benchmark metal-oxo MOFs with the identical organic linker ( e.g . UiO-66(Zr)-NH 2 and MIL-101(Fe)-NH 2 ) as well 13 , 31 .…”
Section: Introductionmentioning
confidence: 99%
“…The performance is also higher than many benchmark metal-oxo MOFs with the identical organic linker ( e.g . UiO-66(Zr)-NH 2 and MIL-101(Fe)-NH 2 ) as well 13 , 31 .…”
Section: Introductionmentioning
confidence: 99%
“…5d. 52,53 The optical characterization of the prepared photocatalysts can be performed by UV-visible diffuse reflectance spectroscopy (DRS). As shown in the absorption spectra of several photocatalysts in Fig.…”
Section: Resultsmentioning
confidence: 99%
“…[13][14][15][16][17][18] Recently, sustainable green nano adsorbents, 19 and sustainable photocatalytic membranes 20 have been used for water and wastewater remediation of pharmaceuticals. Metal-organic frameworks (MOFs) attracted large attention due to their applications in energy generation, 21 catalytic degradation, 22 gas storage, 23,24 gas/heavy metal adsorption, [25][26][27] chemical catalysis, 28 and environmental remediation. [29][30][31] Even though the bare MOFs can be used as adsorbents, nevertheless, certain disadvantages impede the removal efficiencies for pollutants due to weaker adsorption affinity resulting from their large amount of void space and the limited unsaturated metallic centers.…”
Section: Introductionmentioning
confidence: 99%