robotics. [9,10] More recently, the emergence of analogous platforms that dynamically modulate the propagation of IR radiation (i.e., heat) has facilitated exciting proof-of-principle demonstrations in areas such as energy conservation, [11,12] thermal management, [13,14] and IR camouflage. [15,16] Within this context, devices or systems that can potentially manipulate light across both the visible (400-740 nm) and IR (740 nm to 15 µm) spectral regions remain quite rare. To date, relatively few classes of these technologies have been reported, such as thermochromic phase-change materials, [17][18][19][20] electrochromic devices, [21][22][23] IR-reflecting platforms, [24,25] and reconfigurable soft machines [9] (see Table S1, Supporting Information), and they have featured drawbacks that include a limited degree of spectral modulation, impractical actuation requirements, poor stability to repeated actuation, slow response times, and/or complicated fabrication. [9,[17][18][19][20][21][22][23][24][25] Indeed, the engineering of devices and systems with tandem adaptive functionality across a broad spectral window (i.e., encompassing the visible, near-IR, short-wavelength IR, mid-wavelength IR, and long-wavelength IR) has proven challenging, in part because of the order of magnitude difference in the length scales associated with the propagation of visible and long-wavelength IR light. Consequently, there exists an impetus for the development of advanced multimodal camouflage platforms, which can present new scientific and technological opportunities across multiple fields.Some of the most prominent and impressive examples of soft, deformable systems that can reversibly and precisely change their appearance are found in nature-they are animals called coleoid cephalopods, [26][27][28][29][30][31][32] such as the Japetella heathi pelagic octopus (Figure 1A) [28] and the Taonius borealis glass squid ( Figure 1B). [29,30] These animals are capable of stunning feats of concealment, which include changing the transparency of their bodies by means of a sophisticated skin architecture that controls the transmission, absorption, and reflection of light ( Figure 1C). [26][27][28][29][30][31][32] In its most general form, the skin consists of multiple layers containing pigmented sizechanging organs called chromatophores, [33][34][35] typically narrowband-reflecting cells called iridophores, [36][37][38] and broadbandreflecting cells called leucophores [39][40][41] (Figure 1C). Although their precise arrangement and optical functionalities tend to Soft, mechanically deformable materials and systems that can, on demand, manipulate light propagation within both the visible and infrared (IR) regions of the electromagnetic spectrum are desirable for applications that include sensing, optoelectronics, robotics, energy conservation, and thermal management. However, the development of such technologies remains exceptionally difficult, with relatively few examples reported to date. Herein, this challenge is addressed by engineering ceph...