Fe-containing intermetallics are often detrimental to the mechanical properties in aluminum alloy. However, an Al-Fe alloy system can form an Al þ AlFe eutectic structure in a narrow freezing range, providing the fine Al 13 Fe 4 or Al 6 Fe intermetallics. Herein, the ternary Al-Mg-Fe alloy is selected to achieve the Al þ AlFe eutectic structure composition and form fine AlFe intermetallics for improving the strength and ductility of Al-Mg cast alloy. The results show that as the composition of Al-Mg-Fe alloy is closer to the Al þ AlFe eutectic composition, the amount of coarse Al 13 Fe 4 intermetallics decreases, whereas the amount of fine Al þ Al 13 Fe 4 eutectic increases. The microstructural evolution results in the improvement of yield strength (72.8-92.4 MPa), tensile strength (126.1-213.7 MPa), and the elongation (2.5-6.2%). This work provides a new strategy to improve the mechanical properties in Al-Mg cast alloy.