2005
DOI: 10.1103/physrevb.72.085409
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Structure and lattice dynamics ofSr2CuO2Cl2(001)studied by helium-a

Abstract: Structure and lattice dynamics of the (001) surface of Sr2CuO2Cl2 have been studied by helium atom scattering (HAS). Analysis of diffraction patterns obtained by elastic HAS revealed a surface periodicity consistent with bulk termination, and confirms that the surface is non-polar and stable which favors a SrCl surface termination. Bulk and surface lattice dynamical calculations based on the shell-model were carried out to characterize the experimental phonon dispersions obtained by inelastic HAS. No experimen… Show more

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Cited by 8 publications
(9 citation statements)
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“…The scattered He beam was collected by an angle-resolved detector mounted on a two-axis goniometer, which allows the scattered angle θ f to be varied independently from θ i [31], and allows in-and out-of the scattering-plane measurements. As shown in figure 8, the detector is comprised of an electron gun and a multichannel plate (MCP) electron multiplier [32].…”
Section: Scattered Beam Detection Techniquementioning
confidence: 99%
See 1 more Smart Citation
“…The scattered He beam was collected by an angle-resolved detector mounted on a two-axis goniometer, which allows the scattered angle θ f to be varied independently from θ i [31], and allows in-and out-of the scattering-plane measurements. As shown in figure 8, the detector is comprised of an electron gun and a multichannel plate (MCP) electron multiplier [32].…”
Section: Scattered Beam Detection Techniquementioning
confidence: 99%
“…j . The electron-phonon interaction can be generically written as We now proceed to represent the interaction Hamiltonian (31) in Fourier space. This is achieved by expressing:…”
Section: Hamiltonian Of the Electron-phonon Interacting Systemmentioning
confidence: 99%
“…One can postulate that the 4/m distortion only occurs at the surface. However, surface-sensitive Heatom scattering [23] and angle-resolved photoemission spectroscopy measurements [24] on Sr 2 CuO 2 Cl 2 show no signs of (001) surface reconstruction or unit cell enlargement. Even if the mirror planes are somehow broken at the surface, it still cannot explain our data because ED SHG from the surface of a 4/m structure is forbidden in the SS channel [19].…”
Section: (B)]mentioning
confidence: 91%
“…But x-ray mag-netic circular dichroism measurements on Sr 2 CuO 2 Cl 2 detect no out-of-plane spin canting [26], in keeping with its reported structure that forbids DM interactions. Surface spin canting also seems unlikely given the absence of surface reconstruction [23,24]. Furthermore, in the spontaneous spin canting scenario, one might expect to find a spatial distribution of time-reversed domains characterized by ±Φ that can also flip upon thermal cycling across T N .…”
Section: (B)]mentioning
confidence: 99%
“…The experimental setup and procedures of the HAS measurements are described in details in Ref. [16,18].…”
mentioning
confidence: 99%