“…Unfortunately, natural wollastonite is mainly composed of β-CS with lower carbonation activity. The dissolution of silicate minerals during the carbonation process is a rate-limiting step, , and many physical and chemical methods can accelerate the dissolution of β-CS, e.g., the use of acidic solvents, mechanical grinding, and high temperature treatments. , However, most of these methods either produce secondary waste or increase energy consumption and carbon footprints. In addition, the carbonation of wollastonite produces mainly calcite and silicate gel.…”