microscale actuation. However, these material-based actuators are often slow or only expand or contract axially, preventing use in applications that require volumetric expansions. To address such limitations of existing actuating materials, actuators based on the liquid-to-gas phase change of solvent inclusions encapsulated in a hyperelastic matrix have been realized. Phasechange actuators are capable of inducing rapid volumetric expansion similar to fluidic actuators, without being tethered to an external fluid source. [29][30][31][32] Accepting the advantages of phasechange actuators, we now turn our attention to granular media. Granular assemblies, consisting of discrete grains, can be tuned to accomplish a variety of different responses. For example, favorable self-assembly of granular media can be achieved via modulating interparticle interactions and external stimuli, [33][34][35][36] and granular assemblies with different packing configurations have been shown to yield different bulk properties. [36][37][38][39] Furthermore, granular media can exhibit optimized changes in stiffness during jamming transitions, enabling tunable moduli. [16,[40][41][42][43][44] When unjammed, the bulk material is compliant, and when jammed, the bulk material can achieve the stiffness of the grains. Finally, when mixed into carrier fluids, granular media can impart thixotropic behavior on the carrier fluid due to dynamic jamming, [45][46][47][48] enabling 3D printing of previously unprintable materials. With all the advantageous properties granular media has to offer, the technology has seen application in soft robotics, [49][50][51][52] medical devices, [53][54][55] flexible airfoils, [56] and programmable aggregate architecture. [57] Here, we bring together the unique advantages of phasechange soft actuators and granular media to introduce soft granular actuators made of discrete, volumetrically expanding grains. A single active grain consists of multiple solvent cores encapsulated in a hyperelastic silicone shell (Ecoflex 00-30). At elevated temperatures, the encapsulated solvent vaporizes and increases the internal pressure of the hyperelastic shell, inducing volumetric expansion of the grain. The grains are independently capable of rapid, high-force microscopic actuation, and are also easily arranged into granular assemblies to form larger-scale bulk actuators. Furthermore, agglomerates of active grains can self-assemble from disordered arrangements to conform around objects and exhibit variable moduli. Finally, the use of grains suspended in a carrier solvent or resin enables compatibility with granular self-assembly and 3D printing techniques, offering the potential to print volumetrically expanding actuators into freeform patterns across scales.Recent work has demonstrated the potential of actuators consisting of bulk elastomers with phase-changing inclusions for generating high forces and large volumetric expansions. Simultaneously, granular assemblies have been shown to enable tunable properties via different packing...