“…Especially, their second-order nonlinear susceptibilities, χ (2) , are one or two orders of magnitude larger than those of typical second-order nonlinear materials such as LiNbO 3 and KTP [26,27]. Furthermore, their absorption coefficient in the THz region is several times smaller than that of LiNbO 3 [28]. It is well known that, in the anisotropic birefringent crystals, the input pump and signal waves, and , for difference frequency mixing, and the generated THz wave, , are generally all in the same transmission window of the nonlinear crystal.…”