Accumulative roll bonding (ARB) technique is used to manufacture fine-grained and high-strength Mg-8Li-3Al-1Zn alloy. Then, investigate the microstructure and mechanical properties. Results show that, the ARB-processed sheet possesses good bonding performance. The ARB refines the grains and causes the phase distribution to be scattered. With the increase of ARB passes, the s 0.2, s b , and hardness values are enhanced, whereas the elongation value first decreases, then slightly increases with the increase of ARB passes. The ARB5 sheet possesses the smallest grain size (about 3 mm) and the best comprehensive mechanical properties, the tensile strength, elongation, and hardness are 287.02 MPa, 12.5%, and 77.2 HV 0.05 , respectively.