Clouds developing in a polluted environment tend to have more numerous but smaller droplets. This property may lead to suppression of precipitation and longer cloud lifetime. Absorption of incoming solar radiation by aerosols, however, can reduce the cloud cover. The net aerosol effect on clouds is currently the largest uncertainty in evaluating climate forcing. Using large statistics of 1-km resolution MODIS (Moderate Resolution Imaging Spectroradiometer) satellite data, we study the aerosol effect on shallow water clouds, separately in four regions of the Atlantic Ocean, for June through August 2002: marine aerosol (30°S-20°S), smoke (20°S-5°N), mineral dust (5°N-25°N), and pollution aerosols (30°N-60°N). All four aerosol types affect the cloud droplet size. We also find that the coverage of shallow clouds increases in all of the cases by 0.2-0.4 from clean to polluted, smoky, or dusty conditions. Covariability analysis with meteorological parameters associates most of this change to aerosol, for each of the four regions and 3 months studied. In our opinion, there is low probability that the net aerosol effect can be explained by coincidental, unresolved, changes in meteorological conditions that also accumulate aerosol, or errors in the data, although further in situ measurements and model developments are needed to fully understand the processes. The radiative effect at the top of the atmosphere incurred by the aerosol effect on the shallow clouds and solar radiation is ؊11 ؎ 3 W͞m 2 for the 3 months studied; 2͞3 of it is due to the aerosolinduced cloud changes, and 1͞3 is due to aerosol direct radiative effect.cloud cover ͉ cloud height ͉ indirect effect ͉ radiative forcing ͉ air quality D uring June through August, the Atlantic Ocean is covered by varying concentrations of several aerosol types, each covering a separate latitude belt (see Fig. 1). The Southern Tropical Atlantic (30°S-20°S) is dominated by clean maritime air. The region between 20°S and 5°N is a relatively well defined region covered by smoke from biomass burning in Africa (1, 2). The Northern Tropical Atlantic (5°N-30°N) is under heavy influx of dust from Africa (3), and the Northern Atlantic (30°N-60°N) is impacted by anthropogenic pollution aerosol from North America and Europe. These aerosols absorb and reflect solar radiation to space (4), thereby affecting the regional atmospheric energy balance. Clouds that form in air laden with high aerosol concentrations tend to contain more numerous but smaller droplets that reflect sunlight and cool the Earth (5). The smaller cloud droplets reduce the efficiency of droplet growth by collision coalescence, which at least under some conditions (6) reduce precipitation formation and increase cloud lifetime (7,8). However, there is a second pathway for aerosols to affect clouds: Smoke, pollution, and dust aerosols absorb solar radiation, heat the atmosphere, and reduce evaporation from the surface (9-11). As a result, smoke over the Amazon or pollution aerosol over the Indian Ocean can inhibit cloud...