“…Therefore, the toughening of nanostructured metals has aroused the interest of researchers. In the recent 20 years, in order to improve their ductility, researchers have multilevel-constructed the composition, size, and distribution of different nanostructures, and some significant achievements have been made: (1) the bimodal structure is the introduction of a certain volume of micron-leveled coarse grains into the nanograined metal, and the resulting metal has the strength of the nanograined metal and the plasticity of the coarse-grained metal, i.e., good mechanical properties [ 17 , 18 , 19 , 20 ]; (2) by introducing nanotwinned (NT) structure inside the grains, the metal exhibits excellent mechanical properties, including high strength, plasticity, work-hardening rate, and fatigue performance, due to the relatively low interface energy and coherent characteristics of twin boundaries (TBs) [ 21 , 22 , 23 , 24 ]; (3) microstructure in which grain size, structure, and/or composition continuously change from nanometer-scale to micrometer-scale, i.e., a gradient nanostructure, has the performance advantages of each scale structure, so as to simultaneously realize strengthening and toughening [ 25 , 26 , 27 , 28 ]; (4) the supra-nano-dual-phase (SNDP) nanostructure consists of two phases with differences in structure or composition, i.e., heterogeneous two-phase nanostructure, and not only exhibits excellent mechanical properties, but also presents other functional properties, such as soft magnetic properties and thermal stability [ 29 , 30 ].…”