We have performed X-ray diffraction (XRD) and AC magnetic susceptibility measurements on polycrystalline LaMn 2-x Ni x Si 2 (0.0 ≤ x ≤ 2.0) silicides for magnetic characterization in fields of about a few Oe at a temperature range 15 -325 K. All compounds crystallize in the naturally layered ThCr 2 Si 2 -type structure with the space group I4/mmm. Substitution of Ni for Mn leads to a linear decrease in the lattice constant c and the unit cell volume, while it gives rise to a change of magnetic properties from ferromagnetic to antiferromagnetic behavior for small values of x < 1. The sample with x = 0.8 has a Néel temperature of about 35 K, associated with anti-ferromagnetic behavior. However, for x = 1, anti-ferromagnetic behavior is diminished and paramagnetic behavior becomes dominant. For x = 2, the sample becomes virtually nonmagnetic. The samples with x ≤ 0.5 exhibit mixed magnetic properties composed of ferromagnetic and anti-ferromagnetic interactions, below the Curie temperature T C (Mn). The results are collected in the magnetic phase diagram.