2019
DOI: 10.1039/c9fd90012h
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Theory of hot electrons: general discussion

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Cited by 41 publications
(42 citation statements)
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“…47 The oscillatory population and depopulation of these states indicate that they would not likely be individually separable while they are a part of the plasmon as Coulomb interaction is an essential part of the excitation. 48 The resonant transitions have zero Coulomb energy contribution and the occupations of the corresponding electron and hole states grow steadily as the plasmon decays (Fig. 2c; solid lines).…”
Section: Resultsmentioning
confidence: 93%
See 1 more Smart Citation
“…47 The oscillatory population and depopulation of these states indicate that they would not likely be individually separable while they are a part of the plasmon as Coulomb interaction is an essential part of the excitation. 48 The resonant transitions have zero Coulomb energy contribution and the occupations of the corresponding electron and hole states grow steadily as the plasmon decays (Fig. 2c; solid lines).…”
Section: Resultsmentioning
confidence: 93%
“… 49 The oscillatory population and depopulation of these states indicate that they would not likely be individually separable while they are a part of the plasmon as the Coulomb interaction is an essential part of the excitation itself. 50 …”
Section: Resultsmentioning
confidence: 99%
“…In direct and hybrid plasmonic photocatalysis, it is important to distinguish between electron‐ and heat‐driven photochemistry. [ 118,192–196 ] Christopher et al. have proposed that the trend of the photocatalytic rate as a function of incident light intensity and kinetic isotopic effects (KIEs) can be used to make this distinction.…”
Section: Lspr‐mediated Pathways Responsible For Photocatalytic Enhancement On Hpnsmentioning
confidence: 99%
“…As extensively discussed in the literature, an accurate description of the optical phenomena occurring in plasmonic nanostructures requires the electron excitation to be dealt with from different perspectives, [ 22–25 ] such as the quasi‐classical description [ 26 ] (including the Drude model and the kinetic Boltzmann approach) and the quantum formalism. [ 27 ] In particular, quantum effects have to be accounted for when describing the generation of high‐energy nonthermal electrons.…”
Section: Introductionmentioning
confidence: 99%
“…quickly collide and exchange their energies with many lowerenergy electrons (electron thermalization) producing a thermalized electron distribution characterized by an overall increased electron temperature. [19][20][21] As extensively discussed in the literature, an accurate description of the optical phenomena occurring in plasmonic nanostructures requires the electron excitation to be dealt with from different perspectives, [22][23][24][25] such as the quasi-classical description [26] (including the Drude model and the kinetic Boltzmann approach) and the quantum formalism. [27] In particular, quantum effects have to be accounted for when describing the generation of high-energy nonthermal electrons.…”
Section: Introductionmentioning
confidence: 99%