2013
DOI: 10.1103/physrevb.88.115128
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Thermoelectric effect of correlated metals: Band-structure effects and the breakdown of Mott's formula

Abstract: We study the thermoelectric effect of two-dimensional metals on a square lattice within semiclassical Boltzmann transport theory with particular focus on electron-electron scattering. We compute the electrical conductivity and the Seebeck coefficient as a function of band filling and temperature for generically chosen hopping parameters in a two-dimensional tight binding model. The Boltzmann equation is solved numerically after computing the full collision integral taking the angular and radial degrees of free… Show more

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Cited by 27 publications
(23 citation statements)
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“…Finally, we consider the possibility that a Lifshitz transition might account for transport and thermopower behaviors near p c1 . A Lifshitz transition, which does reconstruct the FS, under certain circumstances can produce a jump and sign change in S/T as a function of some non-thermal control parameter that tunes the chemical potential 37 or magnetic exchange. 38 Though these theoretical models 37,38 may capture aspects of our experimental observations, presently it is not possible to compare directly predictions of these models to our results as a function of pressure.…”
Section: Discussionmentioning
confidence: 99%
“…Finally, we consider the possibility that a Lifshitz transition might account for transport and thermopower behaviors near p c1 . A Lifshitz transition, which does reconstruct the FS, under certain circumstances can produce a jump and sign change in S/T as a function of some non-thermal control parameter that tunes the chemical potential 37 or magnetic exchange. 38 Though these theoretical models 37,38 may capture aspects of our experimental observations, presently it is not possible to compare directly predictions of these models to our results as a function of pressure.…”
Section: Discussionmentioning
confidence: 99%
“…While the oscillations may indeed be related to those seen in [18], there have recently been several theoretical reports describing situations where the Mott relation (equation (1)) breaks down. These include the vicinity of a quantum critical point [19], proximity to a Lifshitz transition [20], and, remarkably, even far away from a critical point [21].…”
Section: Discussionmentioning
confidence: 99%
“…[36,38], the side of the transition where the new pocket is absent and where the neck is not broken corresponds to region I. Figures 4(a)-4(d) present theoretical predictions for the signatures one expects to observe in electrical conductivity σ and thermopower at a LT of a three-dimensional band [36,38,39]. E c − E F defines the distance of the extremum in the band structure to the Fermi energy.…”
mentioning
confidence: 99%