Infrared Dark Clouds (IRDCs) harbor the earliest phases of massive star formation, and many of the compact cores in IRDCs, traced by millimeter continuum or by molecular emission in high critical density lines, host massive young stellar objects (YSOs). We used the Robert C. Byrd Green Bank Telescope (GBT) and the Karl G. Jansky Very Large Array (VLA) to map NH 3 and CCS in nine IRDCs to reveal the temperature, density, and velocity structures and explore chemical evolution in the dense (> 10 22 cm −2 ) gas. Ammonia is an excellent molecular tracer for these cold, dense environments. The internal structure -2and kinematics of the IRDCs include velocity gradients, filaments, and possibly colliding clumps that elucidate the formation process of these structures and their YSOs. We find a wide variety of substructure including filaments and globules at distinct velocities, sometimes overlapping at sites of ongoing star formation. It appears that these IRDCs are still being assembled from molecular gas clumps even as star formation has already begun, and at least three of them appear consistent with the morphology of "hub-filament structures" discussed in the literature. Furthermore, we find that these clumps are typically near equipartition between gravitational and kinetic energies, so these structures may survive for multiple free-fall times.University Galactic Ring Survey (BU-GRS) , and thus determined velocities, kinematic distances, and physical properties of the population of clouds. The darkest clouds have very high column densities, as high as approximately 10 24 -10 25 cm −2 .The terms "core" and "clump" are frequently used in the literature, but the meanings are not standardized. We use the term "core" to refer to an unresolved or marginally resolved overdense structure <0.1 pc across and tens of solar masses. We then use the term "clump" to refer to a resolved structure (e.g. projected area greater than three times the area of the beam) within an IRDC and is assigned by a clump deconvolution algorithm (see §4.1 for description of algorithms used). "Average" results of spectral line fitting presented in this paper are averaged over clumps. We also occasionally refer to the velocity components within IRDCs when the IRDC's emission primarily occurs at two or more distinct velocities with little emission at the intermediate velocities; a velocity component may have one or more clump associated with it.