“…Millimeter-wave technology with its extremely wide frequency band (B135 GHz, considering the atmospheric window), high resolution, low delay (less than 1 ms) and excellent transmission stability, has shown many advantages in current and future wireless communication systems, such as 5G (the 5th generation mobile communication technology), weapons guidance, radar systems and other military and civilian fields. [1][2][3][4][5][9][10][11][12] Correspondingly, to achieve high-performance of passive devices and reduce the power consumption problems from the increasing frequency, the dielectric performance of microwave dielectric ceramics (MWDCs) should be further optimised. In practical applications, the performance parameters of MWDCs should satisfy the following criteria: (a) a low dielectric loss (tan d), signifying a higher Q Â f value (Q E 1/tan d) to reduce signal damping; (b) a suitable dielectric constant (e r ) to match different device applications; (c) a near-zero temperature coefficient of the resonant frequency (t f ) to ensure thermal stability.…”