Cu/A5052 dissimilar metal laminates (DMLs) were fabricated by an accumulative roll bonding process. The Cu/A5052 DML consisted of hard and soft layers, in other words, high and low shear modulus layers, which is called a mille-feuille structure (MFS). The Cu/A5052 DML with the MFS showed kink deformation during monotonic compression. Kink formation was analyzed by in-situ optical microscopy and digital image correlation. The development behavior and morphology of the ortho-type kink depended on the annealing conditions prior to the compression tests. Based on the observations and measurements, criteria for kink formation in the DML with the MFS were proposed.