Abstract. We investigate the impact of model trace gas transport schemes on the
representation of transport processes in the upper troposphere and lower
stratosphere.
Towards this end, the Chemical Lagrangian Model of the Stratosphere (CLaMS)
was coupled to the ECHAM/MESSy Atmospheric Chemistry (EMAC) model
and results from the two transport schemes (Lagrangian critical Lyapunov
scheme and flux-form semi-Lagrangian, respectively) were compared.
Advection in CLaMS was driven by the EMAC simulation winds, and
thereby the only differences in transport between the two sets of
results were caused by differences in the transport schemes.
To analyze the timescales of large-scale transport, multiple
tropical-surface-emitted tracer pulses were performed to calculate age of
air spectra, while smaller-scale transport was analyzed via idealized,
radioactively decaying tracers emitted in smaller regions (nine
grid cells) within the stratosphere.
The results show that stratospheric transport barriers are significantly
stronger for Lagrangian EMAC-CLaMS transport due to reduced numerical
diffusion.
In particular, stronger tracer gradients emerge around the polar
vortex, at the subtropical jets, and at the edge of the tropical
pipe.
Inside the polar vortex, the more diffusive EMAC flux-form semi-Lagrangian
transport scheme results in a substantially higher amount of air with ages
from 0 to 2 years (up to a factor of 5 higher).
In the lowermost stratosphere, mean age of air is much smaller in EMAC,
owing to stronger diffusive cross-tropopause transport.
Conversely, EMAC-CLaMS shows a summertime lowermost stratosphere
age inversion – a layer of older air residing below younger air
(an “eave”).
This pattern is caused by strong poleward transport above the
subtropical jet and is entirely blurred by diffusive
cross-tropopause transport in EMAC.
Potential consequences from the choice of the transport scheme on
chemistry–climate and geoengineering simulations are discussed.