The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase was first predicted in 2D superconductors about 50 years ago, but so far unambiguous experimental evidences are still lacked. The recently experimentally realized spin-imbalanced Fermi gases may potentially unveil this elusive state, but require very stringent experimental conditions. In this Letter, we show that FFLO phases may be observed even in a 3D degenerate Fermi gas with spin-orbit coupling and in-plane Zeeman field. The FFLO phase is driven by the interplay between asymmetry of Fermi surface and superfluid order, instead of the interplay between magnetic and superconducting order in solid materials. The predicted FFLO phase exists in a giant parameter region, possesses a stable long-range superfluid order due to the 3D geometry, and can be observed with experimentally already achieved temperature (T ∼ 0.05EF ), thus opens a new fascinating avenue for exploring FFLO physics. The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase, characterized by Cooper pairs with finite total momentum and spatially modulated order parameters, was predicted to exist in certain region of 2D superconductors in high Zeeman fields [1][2][3]. This fascinating state arises from the interplay between magnetic and superconducting order, and now is a central concept for understanding many exotic phenomena in different physics branches [4][5][6][7][8][9][10][11][12]. Despite tremendous experimental and theoretical efforts in the past five decades, there is still no unambiguous experimental evidence for FFLO states [11]. The experimental difficulty may arise from several different aspects, such as the depairing of Cooper pairs due to orbital or Pauli effects in strong magnetic fields and unavoidable disorder effects in solid state materials.The recent experimental realization of spin-imbalanced Fermi gases [13][14][15][16][17] provides a new excellent platform for exploring FFLO physics. In Fermi gases, the effective Zeeman field is generated through the population imbalance between two spins, therefore the orbital effects (e.g., vortices induced by the magnetic field) are absent even in 3D. The Fermi gases are also free of disorder and all experimental parameters are highly controllable. These advantages have sparked tremendous recent interest in exploring FFLO physics in spin-imbalanced Fermi gases [18][19][20][21][22][23][24][25][26][27][28]. However, the FFLO phase only exists in a narrow parameter regime in 3D due to the Pauli depairing effect [18,22,23]. Furthermore, the free energy difference between the FFLO state and the BCS superfluid is extremely small. As a result, only the transition from the BCS superfluid to the normal gas [13][14][15] has been observed in experiments in 3D spin-imbalanced Fermi gases. Current experimental and theoretical efforts on the FFLO state have focused on low dimensions (1D or 2D) [29][30][31][32][33], where quantum and thermal (at finite temperature) fluctuations may become crucial and the physics is much more complicated [34][35][36].In this Lett...