This paper reports a novel ultraviolet (UV) photodetector based on a TiO 2 /graphene hybrid, with high responsivity (0.482 A W −1 ) at 3 V bias and 330 nm irradiation, which is ~100 times higher than that based on pure TiO 2 . The collaboration of TiO 2 and graphene in the hybrid material contributes to the high performance of the device. To be more specific, graphene provides a large surface area to load sufficient TiO 2 nanoparticles, and the generated electrons are instantly collected due to the prominent electrical properties of graphene which can overcome the low quantum efficiency of pristine TiO 2 caused by recombination of photoinduced electron-hole pairs. The device was fabricated on a flexible substrate using a facile spraying method that shows the possibility of broadening the future of photodetectors in wearable devices. An on-board interface circuit based on commercial IC components is implemented to collaborate with the photodetector to demonstrate a UV sensing application.