This article aims to investigate free vibration and buckling of functionally graded (FG) nanoporous metal foam (NPMF) nanoshells. The first-order shear deformation (FSD) shell theory is adopted and the theoretical model is formulated by using Mindlin’s most general strain gradient theory, which can derive several well-known simplified models. The symmetric and unsymmetric nanoporosity distributions are considered for the structural composition. Hamilton’s principle is employed to deduce the governing equations as well as the boundary conditions. Then, via the Navier solution technique, an analytical solution for the free vibration and buckling of FG NPMF nanoshells is presented. Afterwards, a detailed parametric analysis is conducted to highlight the effects of the nanoporosity coefficient, nanoporosity distribution, length scale parameter, and geometrical parameters on the mechanical behaviors of FG NPMF nanoshells.