Phase-specific thermal expansion behavior and mechanical deformation behavior of a directionally solidified NiAl-Cr(Mo) lamellar in situ composite were investigated by using real-time in situ neutron diffraction during compression at elevated temperatures up to 800 o C. Tensile and compressive thermal residual stresses were found to exist in the NiAl phase and Cr ss (solid solution) phase, respectively. Based on the evolution of lattice spacings and phase stresses, the phase-specific deformation behavior was analyzed qualitatively and quantitatively. Estimates of phase stresses were derived by Hooke"s law on the basis of a new method for the determination of stress-free lattice spacing in in situ composites. During compressive loading, the NiAl phase yields earlier than the Cr ss phase. The Cr ss phase carries much higher stress than the NiAl phase, and displays consistent strain hardening at all temperatures. The NiAl phase exhibits strain hardening at relatively low temperatures and softening at high temperatures. During unloading, the NiAl phase yields in tension whereas the Cr ss phase unloads elastically. In addition, post-test microstructural observations show phase-through cracks at room temperature, micro cracks along phase interfaces at 600 o C and intact lamellae kinks at 800 o C, which is assumed as the result of increasing deformability of both phases as temperature rises.