X-ray photoelectron spectroscopy and full potential studies of the electronic density of state of ternary oxyborate Na3La9O3(BO3)8

New nonlinear crystals Na(3)La(9)O(3)(BO(3))(8) (abbreviated as NLBO) with desired morphologies, high quality and weight exceeding 40g have been grown along different directions, such as [001], [110], and [100], by top-seeded solution growth(TSSG) method. The refractive indices were accurately measured over the full transmission range, and the second-order nonlinear optical coefficients were determined by the Maker fringe technique. The optimal phase-matching (PM) conditions and the corresponding effective nonlinear coefficient were calculated for second harmonic generation (SHG) at different wavelengths. In order to confirm the correctness of our calculation, we also performed the SHG experiments under 1064 and 800 nm pumping, respectively. In addition, we directly compared the SHG performance of NLBO with that of LBO under the same experimental conditions with the 1064 nm pumping source. As the results, a conversion efficiency of 58.3% at 532 nm was obtained for NLBO, and whereas only 21.5% was obtained for LBO, indicating that NLBO is a highly attractive nonlinear material for frequency conversion of pulses into the visible and ultraviolet.

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X-ray photoelectron spectroscopy and full potential studies of the electronic density of state of ternary oxyborate Na3La9O3(BO3)8

Cited by 5 publications

References 21 publications

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