Investigations of the spin dynamics of the geometrically frustrated pyrochlore (Tb(p)Y(1-p))2Ti2O7, using muon spin relaxation and neutron spin echo, as a function of magnetic coverage p, have been carried out. Our major finding is that paramagnetic fluctuations prevail as T-->0 for all values of p, and that they are sensitive to dilution, indicating a cooperative spin motion. However, the percolation threshold pc is not a critical point for the fluctuations. We also find that the low temperature spectral density has a 1/f behavior, and that dilution slows down the spin fluctuations.
Muon spin relaxation and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagomé system (CuxZn(1-x))3V2O7(OH)2 2H2O. In the pure x=1 system we found a slowing down of Cu spin fluctuations with decreasing temperature towards T approximately 1 K, followed by slow and nearly temperature-independent spin fluctuations persisting down to T=50 mK, indicative of quantum fluctuations. No indication of static spin freezing was detected in either of the pure (x=1.0) or diluted samples. The observed magnitude of fluctuating fields indicates that the slow spin fluctuations represent an intrinsic property of kagomé network rather than impurity spins.
We report muon spin relaxation (µSR) and magnetization measurements, together with synthesis and characterization, of the Li-intercalated layered superconductors Li x HfNCl and Li x ZrNCl with/without co-intercalation of THF
Muon spin relaxation (µSR) measurements in high transverse magnetic fields ( ĉ) revealed strong field-induced quasi-static magnetism in the underdoped and Eu doped (La,Sr)2CuO4 and La1.875Ba0.125CuO4, existing well above Tc and TN . The susceptibility-counterpart of Cu spin polarization, derived from the muon spin relaxation rate, exhibits a divergent behavior towards T ∼ 25 K. No field-induced magnetism was detected in overdoped La1.81Sr0.19CuO4, optimally doped Bi2212, and Zn-doped YBa2Cu3O7.
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