We report muon spin relaxation (SR) measurements using single crystals of oxygen-intercalated stage-4 La 2 CuO 4.11 ͑LCO:4.11͒ and La 1.88 Sr 0.12 CuO 4 ͑LSCO:0.12͒, in which neutron scattering studies have found incommensurate magnetic Bragg reflections. In both systems, zero-field SR measurements show muon spin precession below the Néel temperature T N with frequency 3.6 MHz at T→0, having a Bessel function line shape, characteristic of spin-density-wave systems. The amplitude of the oscillating and relaxing signals of these systems is less than half the value expected for systems with static magnetic order in 100% of the volume. Our results are consistent with a simulation of local fields for a heuristic model with ͑a͒ incommensurate spin amplitude modulation with the maximum ordered Cu moment size of ϳ0.36 B , ͑b͒ static Cu moments on the CuO 2 planes forming ''islands'' having typical radius 15-30 Å, comparable to the in-plane superconducting coherence length, and ͑c͒ the measured volume fraction of magnetic muon sites V increasing progressively with decreasing temperature below T N towards V ϳ40% for LCO:4.11 and 18% for LSCO:0.12 at T→0. These results may be compared with correlation lengths in excess of 600 Å and a long range ordered moment of 0.15Ϯ0.05 B measured with neutron scattering techniques. In this paper we discuss a model that reconciles these apparently contradictory results. In transverse magnetic field SR measurements, sensitive to the in-plane magnetic field penetration depth ab , the results for LCO:4.11 and LSCO:0.12 follow correlations found for underdoped, overdoped and Zn-doped high-T c cuprate systems in a plot of T c versus the superconducting relaxation rate (T→0). This indicates that the volume-integrated value of n s /m* ͑superconducting carrier density / effective mass͒ is a determining factor for T c , not only in high-T c cuprate systems without static magnetism, but also in the present systems where superconductivity coexists with static spin-densitywave spin order.
We investigate the Néel temperature of Sr 2 CuO 3 as a function of the site dilution at the Cu ͑S =1/2͒ sites with Pd ͑S =0͒, utilizing the muon spin relaxation ͑SR͒ technique. The Néel temperature, which is T N = 5.4 K for the undoped system, becomes significantly reduced for less than one percent of doping Pd, giving a support for the previous proposal for the good one-dimensionality. The Pd concentration dependence of the Néel temperature is compared with a recent theoretical study [S. Eggert, I. Affleck, and M. D. P. Horton, Phys. Rev. Lett. 89, 47 202 (2002)] of weakly coupled one-dimensional antiferromagnetic chains of S =1/2 spins, and a quantitative agreement is found. The inhomogeneity of the ordered moment sizes is characterized by the SR time spectra. We propose a model that the ordered moment size recovers away from the dopant S = 0 sites with a recovery length of Ϸ 150− 200 sites. The origin of the finite recovery length for the gapless S =1/2 antiferromagnetic chain is compared to the estimate based on the effective staggered magnetic field from the neighboring chains.
Muon spin relaxation and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagomé system (CuxZn(1-x))3V2O7(OH)2 2H2O. In the pure x=1 system we found a slowing down of Cu spin fluctuations with decreasing temperature towards T approximately 1 K, followed by slow and nearly temperature-independent spin fluctuations persisting down to T=50 mK, indicative of quantum fluctuations. No indication of static spin freezing was detected in either of the pure (x=1.0) or diluted samples. The observed magnitude of fluctuating fields indicates that the slow spin fluctuations represent an intrinsic property of kagomé network rather than impurity spins.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.