A flexible perovskite solar yarn with an impressive active lifetime (>216 h) and an exceptional photon conversion efficiency is prepared under ordinary conditions. The champion device demonstrates an average linear mass density of 0.89 mg cm−1 and can be bent over a loop diameter of 2.5 mm, with a negligible efficiency loss. Photoactive nanofibers composed of a polyvinylpyrrolidone (PVP) central strain and a perovskite phase on the surface (with average grain size of 275 ± 14.3 nm), are prepared by electrospinning, at 18 kV, relative humidity of 75%, and a temperature of 25 °C. This bilayered configuration promises superior mechanical strength and flexibility, together with an excellent photovoltaic character, compared with their dip coated counterparts. Photoactive perovskite nanofibers are incorporated into a plied‐solar yarn, with an organic hole‐conductive layer, poly(3‐hexylthiophene‐2,5‐diyl)‐coated on silver yarn electrode, and a composite electron conductive layer, phenyl‐C61‐butyric acid methyl ester (PC61BM)‐SnO2 coated on a carbon yarn. An individual double‐twisted solar yarns yields 15.7% champion power conversion efficiency, while a 30.5 mm × 30.5 mm active area of plain‐woven fabric generates a maximum power density of 1.26 mW cm−2 under one sun (1000 W m−2) solar illumination.
Plastic bottles are generally recycled by remolding them into numerous products. In this study, waste from plastic bottles was used to fabricate recycled polyethylene terephthalate (r-PET) nanofibers via the electrospinning technique, and high-performance conductive polyethylene terephthalate nanofibers (r-PET nanofibers) were prepared followed by copper deposition using the electroless deposition (ELD) method. Firstly, the electrospun r-PET nanofibers were chemically modified with silane molecules and polymerized with 2-(methacryloyloxy) ethyl trimethylammonium chloride (METAC) solution. Finally, the copper deposition was achieved on the surface of chemically modified r-PET nanofibers by simple chemical/ion attraction. The water contact angle of r-PET nanofibers, chemically modified r-PET nanofibers, and copper deposited nanofibers were 140o, 80o, and 138o, respectively. The r-PET nanofibers retained their fibrous morphology after copper deposition, and EDX results confirmed the presence of copper on the surface of r-PET nanofibers. XPS was performed to analyze chemical changes before and after copper deposition on r-PET nanofibers. The successful deposition of copper one r-PET nanofibers showed an excellent electrical resistance of 0.1 ohms/cm and good mechanical strength according to ASTM D-638.
Perovskite solar cells connected with other power devices have the potential to drive consumer electronics in the smartest possible way. Here we review the means of integration, materials for integration, and performance of hybrid devices.
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