Across the globe, the quest for clean water is escalating for both households as well as agricultural exigencies. With the industrial revolution and swift population growth, the contamination of natural water bodies has impacted the lives of more than two billion people around the world. A spectrum of water-saving solutions has been examined. Nonetheless, most of them are either energy-inefficient or limited to only a particular region. Thus, the pursuit of clean and potable drinking water is an assignment that invites collective discourse from scientists, policymakers, and innovators. In this connection, the presence of moisture in the atmosphere is considered one of the major sources of potential freshwater. Thus, fishing in atmospheric water is a mammoth opportunity. Atmospheric water harvesting (AWH) by some plants and animals in nature (particularly in deserts or arid regions) at low humidity serves as an inspiration for crafting state-of-the-art water harvesting structures and surfaces to buffer the menace of acute water scarcity. Though a lot of research articles and reviews have been reported on bioinspired structures with applications in water and energy harvesting, the area is still open for significant improvisation. This work will address the multidimensional-based AWH ability of natural surfaces or fabricated structures without the involvement of toxic chemicals. Moreover, the review will discuss the availability of clean technologies for emulating fascinating natural surfaces on an industrial scale. In the end, the current challenges and the future scope of bioinspired water harvesters will be discussed for pushing greener technologies to confront climate change.

Water is indispensable for sustaining life on Earth. Oil−water mixtures/or emulsions from industrial waste and other sources are a serious environmental concern for both human beings and aquatic life. Specially treated meshes and textiles with opposing wettability for oil−water separation have been widely reported as a solution to this challenge. Nonetheless, such membranes are hindered by certain drawbacks, including high manufacturing costs, usage of harmful chemicals, and lack of diverse applicability. Here, we report a facile method to fabricate Janus oil−water separation membrane with a controllable pore structure that has a unique directional flux rate. The superhydrophobic (SHB) layer of the membrane is formed by transfer-printing (TP) carbon soot particles onto a polydimethylsiloxane (PDMS)-coated paper surface. Meanwhile, a spincoated thin layer of chitosan on the other side of the film served as a hydrophilic (SHL) and underwater oleophobic face. A pulsed laser beam is used to produce micropores with conical structures. The separation ability of the membrane for both light oil−water and heavy oil−water mixtures is thoroughly investigated. Moreover, the significance of the pore shape and the size is also elucidated. The flexible Janus membrane showed high thermal stability and ideal (i.e., 99.8%) separation efficiency. The membrane can be produced over a 151 cm 2 size range. Besides having flexibility and superior performance, the fabricated membrane is environmentally friendly and economically viable. This work establishes a scalable basis for efficient and low-cost oil/water membranes from non-porous substrates.