We present a new method for calculating backscatter ratios of the stratospheric sulfate aerosol (SSA) layer from daytime and nighttime lidar measurements. Using this new method we show a first year-round dataset of stratospheric aerosol backscatter ratios at high latitudes. The SSA layer is located at altitudes between the tropopause and about 30 km. It is of fundamental importance for the radiative balance of the atmosphere. We use a state-of-the-art Rayleigh-Mie-Raman lidar at the Arctic Lidar Observatory for Middle Atmosphere Research (ALOMAR) station located in northern Norway (69 • N, 16 • E; 380 m a.s.l.). For nighttime measurements the aerosol backscatter ratios are derived using elastic and inelastic backscatter of the emitted laser wavelengths 355, 532 and 1064 nm. The setup of the lidar allows measurements with a resolution of about 5 min in time and 150 m in altitude to be performed in high quality, which enables the identification of multiple sub-layers in the stratospheric aerosol layer of less than 1 km vertical thickness.We introduce a method to extend the dataset throughout the summer when measurements need to be performed under permanent daytime conditions. For that purpose we approximate the backscatter ratios from color ratios of elastic scattering and apply a correction function. We calculate the correction function using the average backscatter ratio profile at 355 nm from about 1700 h of nighttime measurements from the years 2000 to 2018. Using the new method we finally present a year-round dataset based on about 4100 h of measurements during the years 2014 to 2017.

Abstract. We report on the retrieval of stratospheric aerosol particle size and extinction coefficient profiles from multi-color backscatter measurements with the Rayleigh-Mie-Raman lidar operated at the Arctic Lidar Observatory for Middle Atmosphere Research (ALOMAR) in northern Norway. The retrievals are based on a two-step approach. In a first step the median radius of an assumed log-normal particle size distribution with fixed width is retrieved based on the color ratio formed from the measured backscatter ratios at wavelenghts of 1064 nm and 532 nm. An intrinsic ambiguity of the retrieved aerosol size information is discussed. In a second step, this particle size information is used to convert the measured lidar backscatter ratio to aerosol extinction coefficients. The retrieval is currently based on monthly-averaged lidar measurements covering the period from the year 2000 to present. A sensitivity study is presented that allows establishing an error budged for the aerosol retrievals. Assuming a log-normal aerosol particle size distribution with a geometric width of S = 1.3, median radii on the order of 100 nm are retrieved. The median radii are found to generally decrease with increasing altitude. The retrieved aerosol extinction profiles are compared to observations with various current and past satellite instruments.

We report on the retrieval of stratospheric aerosol particle size and extinction coefficient profiles from multi-color backscatter measurements with the Rayleigh–Mie–Raman lidar operated at the Arctic Lidar Observatory for Middle Atmosphere Research (ALOMAR) in northern Norway. The retrievals are based on a two-step approach. In a first step, the median radius of an assumed monomodal log-normal particle size distribution with fixed width is retrieved based on a color index formed from the measured backscatter ratios at the wavelengths of 1064 nm and 532 nm. An intrinsic ambiguity of the retrieved aerosol size information is discussed. In a second step, this particle size information is used to convert the measured lidar backscatter ratio to aerosol extinction coefficients. The retrieval is currently based on monthly-averaged lidar measurements and the results for March 2013 are discussed. A sensitivity study is presented that allows for establishing an error budget for the aerosol retrievals. Assuming a monomodal log-normal aerosol particle size distribution with a geometric width of S = 1.5, median radii on the order of below 100 nm are retrieved. The median radii are found to generally decrease with increasing altitude. The retrieved aerosol extinction profiles are compared to observations with the OSIRIS (Optical Spectrograph and InfraRed Imager System) and the OMPS-LP (Ozone Mapping Profiling Suite Limb Profiler) satellite instruments in the 60∘ N to 80∘ N latitude band. The extinction profiles that were retrieved from the lidar measurements show good agreement with the observations of the two satellite instruments when taking the different wavelengths of the instruments into account.

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