The micro-luminescence spectra of the diluted magnetic semiconductor (DMS) can reflect the spin-exciton interaction and related relaxation process. Here the micro-photoluminescence (micro-PL) spectra and PL lifetime measurements have been done on an individual ferromagnetic (FM)-coupled cobalt (Co) doped zinc selenide (ZnSe) nanowire. There occurs a double-peak profile in its near bandedge emission spectrum: the first peak is from free exciton (FX) and the second comes from magnetic polaron (MP). In their temperature dependent PL spectra, the MP emission peak demonstrates obviously temperature-independent behavior, in contrast to the behaviors of FX and reported exciton MP in nanobelt. It is found that in this Co(II) doped ZnSe nanowires, this MP's temperature-independent emission is related to the coupling between exciton and a FM nanocluster (↑↑↓). The nanocluster is likely due to the interaction of Se vacancies of the wide bandgap semiconductors with the antiferromagnetic (AFM) arrangement transition metal (TM) ions in these Se-deficient Co doped ZnSe nanowires. These results reflect that the AFM coupling TM ions pair can give rise to FM behavior with the involvement of positive charge defect, also indicating that the micro-luminescence detection can be used to study the magnetic coupling in DMS.
Diluted magnetic semiconductor (DMS) nanostructures are promising platform to modulate carriers and spins for new information devices. Here we report that the high quality pure CH 3 NH 3 PbBr 3 microrods and Mn doped CH 3 NH 3 PbBr 3 microrods have been prepared by solution method and in which the exciton magnetic polarons (EMP) formed in Mn doped microrods, and a single mode lasing phenomenon from collective EMP in single microrod have been detected when excited by fs pulse laser. This finding helps to understand the exciton and spin interactions and pave ways to the realization of new type of bosonic laser.
Assisted by a quantum dot-microcavity coupled system, we propose an entanglement concentration scheme for concentrating two unknown partially entangled three-photon W states into a maximally entangled three-photon W state based on spin selective photon reflection from the cavity and the interference of polarized photons. In the scheme, three parties, say Alice, Bob, and Charlie in different distant locations can successfully share the maximally entangled three-photon W state with a high probability of success by local operations performed by Alice and classical communication. We calculate the probability of success of the scheme and the fidelity of the obtained three-photon W state under practical conditions, whose results show that the scheme can work in both weak coupling and strong coupling regimes.
Co(II) doped ZnTe nanowires are prepared by a thermal evaporation method. The power and temperature dependent micro-photoluminescence spectra of single nanowire demonstrate the double bands near its band edge, and the ferromagnetism behavior for these nanowires is identified. The occurrence of excitonic magnetic polaron (EMP) can account for the second emission band for its higher binding energy and ferromagnetic coupling. This EMP formation in a nanostructure will facilitate to realize magnetic modulation on confined excitons and will find new applications for spinpolarized nanophotonic devices.
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