. Lidar measurements were supplemented with surface-based measurements of PM 2.5 and PM 10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regional sources are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of theÅngström exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of theÅngström exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing.
The variability of total column ozone (TCO) and tropospheric column ozone (TrCO) was examined in Central Asia. Measurements were conducted at the Lidar Station Teplokluchenka in eastern Kyrgyzstan for one year, July 2008-July 2009.TCO was obtained using a handheld Microtops II Ozonometer (TCO-MII) and from the Aura OMI (TCO-OMI) satellite. Nitrogen dioxide (NO 2 ) and formaldehyde concentrations also were obtained from the OMI satellite. Formaldehyde was used as a surrogate for volatile organic compounds. TrCO was estimated by the difference between TCO-OMI and stratospheric column ozone retrieved from the MLS satellite. Comparison of the ground-based TCO-MII with TCO-OMI showed good agreement (r 2 = 0.93), and linear regression between these was used to estimate missing values in the TCO-MII dataset. The contribution of TrCO to TCO varied from 15% in summertime to 5% in winter. High values of TrCO were observed during summer (July: 45 DU) and low values during winter (December: 15 DU), as is typically observed. The average values of TrCO for summer, autumn, winter, and spring were equal to 42, 27, 20, and 30 DU, respectively. Seasonal variability of TrCO corresponded to solar intensity, indicating that TrCO is likely to form through photochemical means rather than stratospheric intrusion.The spatial distribution of NO 2 and VOC were examined to better understand the regional sources of these ozone precursors. Transport from highly populated areas of the Ferghana Valley and Tashkent in Uzbekistan contributed to the TrCO concentrations observed in this work. The HCHO/NO 2 ratio, an indicator of the ozone production rate, suggested that reducing NO 2 would be more effective in reducing TrCO during most of the year, except summer, when reductions of both would likely be needed.
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