Multiferroics have attracted strong interest for potential applications where electric fields control magnetic order. The ultimate speed of control via magnetoelectric coupling, however, remains largely unexplored. Here, we report an experiment in which we drove spin dynamics in multiferroic TbMnO3 with an intense few-cycle terahertz (THz) light pulse tuned to resonance with an electromagnon, an electric-dipole active spin excitation. We observed the resulting spin motion using time-resolved resonant soft x-ray diffraction. Our results show that it is possible to directly manipulate atomic-scale magnetic structures with the electric field of light on a sub-picosecond time scale.

We report on high-field terahertz transients with 0.9-mJ pulse energy produced in a 400  mm² partitioned organic crystal by optical rectification of a 30-mJ laser pulse centered at 1.25 μm wavelength. The phase-locked single-cycle terahertz pulses cover the hard-to-access low-frequency range between 0.1 and 5 THz and carry peak fields of more than 42 MV/cm and 14 Tesla with the potential to reach over 80 MV/cm by choosing appropriate focusing optics. The scheme based on a Cr:Mg₂SiO₄ laser offers a high conversion efficiency of 3% using uncooled organic crystal. The collimated pump laser configuration provides excellent terahertz focusing conditions.

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We present high-power single-cycle carrier-envelope phase locked THz pulses at a central frequency of 2.1 THz with MV/cm electric field strengths and magnetic field strengths beyond 0.3 T. The THz radiation is generated by optical rectification in an organic salt crystal 4-N,N-dimethylamino-4′-N′-methyl stilbazolium tosylate called DAST pumped with the signal wavelength of a powerful optical parametric amplifier. Conversion efficiencies of more than 2% are reported.

The SwissFEL X-ray Free Electron Laser (XFEL) facility started construction at the Paul Scherrer Institute (Villigen, Switzerland) in 2013 and will be ready to accept its first users in 2018 on the Aramis hard X-ray branch. In the following sections we will summarize the various aspects of the project, including the design of the soft and hard X-ray branches of the accelerator, the results of SwissFEL performance simulations, details of the photon beamlines and experimental stations, and our first commissioning results.