Compared with traditional conductive fillers, carbon nanotubes (CNTs) have unique advantages, i.e., excellent mechanical properties, high electrical conductivity and thermal stability. Nanocomposites as piezoresistive films provide an interesting approach for the realization of large area strain sensors with high sensitivity and low manufacturing costs. A polymer-based nanocomposite with carbon nanomaterials as conductive filler can be deposited on a flexible substrate of choice and this leads to mechanically flexible layers. Such sensors allow the strain measurement for both integral measurement on a certain surface and local measurement at a certain position depending on the sensor geometry. Strain sensors based on carbon nanostructures can overcome several limitations of conventional strain sensors, e.g., sensitivity, adjustable measurement range and integral measurement on big surfaces. The novel technology allows realizing strain sensors which can be easily integrated even as buried layers in material systems. In this review paper, we discuss the dependence of strain sensitivity on different experimental parameters such as composition of the carbon nanomaterial/polymer layer, type of polymer, fabrication process and processing parameters. The insights about the relationship between film parameters and electromechanical properties can be used to improve the design and fabrication of CNT strain sensors.

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Abstract. A highly flexible, piezoresistive sensor matrix based on a carbon nanotube (CNT) polymer composite is developed for pressure distribution measurement applications. With an overall height of about 400 µm, the sensors can measure pressure directly, without any deformation elements, such as a cantilever or a deformation membrane. The measurement range is from 2.5 to 640 kPa. Both the position and the pressure of the applied load can be measured and visualized as a resistance change. The relative resistance measurement deviation of the data acquisition system is lower than 3 % for the resistance range of 610Ω to 380 kΩ. This corresponds to a systematic deviation of pressure measurement of less than 3 % in the measurement range. Besides the measurement of pressure, different sizes of loads can be detected as well. The developed fast and compact measurement system allows dynamic pressure measurement, such as gait analysis when used in an insole application.

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