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In article 1400093 H.-Y. Chen and co-workers demonstrate that vapor-based thiol-reactive coatings which are composed of maleimide and vinyl anchoring groups can effectively tailor surface properties through specific conjugation reactions. Thermal stability tests and mechanical adhesion tests have shown robustness for these coatings on various substrates. Suppressed protein fouling property and controlled endothelial cell attachment is demonstrated by using the advanced coating technique.