Abstract. Airborne lidar and in-situ measurements of aerosols and trace gases were performed in volcanic ash plumes over Europe between Southern Germany and Iceland with the Falcon aircraft during the eruption period of the Eyjafjalla 1 volcano between 19 April and 18 May 2010. Flight planning and measurement analyses were supported by a refined Meteosat ash product and trajectory model analysis. The volcanic ash plume was observed with lidar directly over the volcano and up to a distance of 2700 km downwind, and up to 120 h plume ages. Aged ash layers were between a few 100 m to 3 km deep, occurred between 1 and 7 km altitude, and were typically 100 to 300 km wide. Particles collected by impactors had diameters up to 20 µm diameter, with size and age dependent composition. Ash mass concentrations were derived from optical particle spectrometers for aCorrespondence to: U. Schumann (ulrich.schumann@dlr.de) 1 Also known as Eyjafjallajökull or Eyjafjöll volcano, http://www.britannica.com/EBchecked/topic/1683937/ Eyjafjallajokull-volcano particle density of 2.6 g cm −3 and various values of the refractive index (RI, real part: 1.59; 3 values for the imaginary part: 0, 0.004 and 0.008). The mass concentrations, effective diameters and related optical properties were compared with ground-based lidar observations. Theoretical considerations of particle sedimentation constrain the particle diameters to those obtained for the lower RI values. The ash mass concentration results have an uncertainty of a factor of two. The maximum ash mass concentration encountered during the 17 flights with 34 ash plume penetrations was below 1 mg m −3 . The Falcon flew in ash clouds up to about 0.8 mg m −3 for a few minutes and in an ash cloud with approximately 0.2 mg m −3 mean-concentration for about one hour without engine damage. The ash plumes were rather dry and correlated with considerable CO and SO 2 increases and O 3 decreases. To first order, ash concentration and SO 2 mixing ratio in the plumes decreased by a factor of two within less than a day. In fresh plumes, the SO 2 and CO concentration increases were correlated with the ash mass concentration. The ash plumes were often visible slantwise as faint dark layers, even for concentrations below 0.1 mg m −3 .Published by Copernicus Publications on behalf of the European Geosciences Union. U. Schumann et al.: Airborne observations of the Eyjafjalla volcano ash cloud over EuropeThe large abundance of volatile Aitken mode particles suggests previous nucleation of sulfuric acid droplets. The effective diameters range between 0.2 and 3 µm with considerable surface and volume contributions from the Aitken and coarse mode aerosol, respectively. The distal ash mass flux on 2 May was of the order of 500 (240-1600) kg s −1 . The volcano induced about 10 (2.5-50) Tg of distal ash mass and about 3 (0.6-23) Tg of SO 2 during the whole eruption period. The results of the Falcon flights were used to support the responsible agencies in their decisions concerning air traffic in the presence of v...

Airborne measurements of Lidar backscatter, aerosol concentrations (particle diameters of 4 nm to 50 μm), trace gas mixing ratios (SO₂, CO, O₃, H₂O), single particle properties, and meteorological parameters have been performed in volcanic ash plumes with the Falcon aircraft operated by Deutsches Zentrum für Luft- und Raumfahrt (DLR). A series of 17 flights was performed over Europe between Southern Germany and Iceland during the eruption period of the Eyjafjalla¹ volcano between 19 April and 18 May 2010. Flight planning and measurement analyses were supported by a refined Meteosat ash product and trajectory model analysis. The volcanic ash plume was observed with Lidar directly over the volcano and up to a distance of 2700 km downwind. Lidar and in-situ measurements covered plume ages of 7 h to 120 h. Aged ash layers were between a few 100 m to 3 km deep, occurred between 1 and 7 km altitude, and were typically 100 to 300 km wide. Particles collected by impactors had diameters up to 20 μm diameter, with size and age dependent composition. Ash mass concentration was evaluated for a material density of 2.6 g cm^&minus;3 and for either weakly or moderately absorbing coarse mode particles (refractive index 1.59+0<i>i</i> or 1.59+0.004<i>i</i>). In the absorbing case, the ash concentration is about a factor of four larger than in the non-absorbing limit. Because of sedimentation constraints, the smaller results are the more realistic ones for aged plumes. The Falcon flew in ash clouds up to about 1 mg m^&minus;3 for a few minutes and in an ash cloud with more than 0.2 mg m^&minus;3 mean-concentration for about one hour without engine damages. In fresh plumes, the SO₂ concentration was correlated with the ash mass concentration. Typically, 0.5 mg m^&minus;3 ash concentration was related to about 100 nmol mol^&minus;31 SO₂ mixing ratio and 70 nmol mol^&minus;1 CO mixing ratio increases for this volcano period. In aged plumes, layers with enhanced coarse mode particle concentration but without SO₂ enhancements occurred. To first order, ash concentration and SO₂ mixing ratio in the plumes decreased by a factor of two within less than a day. The ash plumes were often visible as faint dark layers even for concentrations below 0.1 mg m^&minus;3. The ozone concentrations and the humidity inside the plumes were often reduced compared to ambient values. The large abundance of volatile Aitken mode particles suggests nucleation of sulfuric acid droplets. Ammonium sulfate particles were also found on the impactors. The effective diameters decreased from about 5 μm in the fresh plume to about 1 μm for plume ...

On 4 July 2014, during the Deep Propagating Gravity Wave Experiment (DEEPWAVE), strong low‐level horizontal winds of up to 35 m s−1 over the Southern Alps, New Zealand, caused the excitation of gravity waves having the largest vertical energy fluxes of the whole campaign (38 W m−2). At the same time, large‐amplitude mesospheric gravity waves were detected by the Temperature Lidar for Middle Atmospheric Research (TELMA) located at Lauder (45.0°S, 169.7°E), New Zealand. The coincidence of these two events leads to the question of whether the mesospheric gravity waves were generated by the strong tropospheric forcing. To answer this, an extensive data set is analyzed, comprising TELMA, in situ aircraft measurements, radiosondes, wind lidar measurements aboard the DLR Falcon as well as Rayleigh lidar and advanced mesospheric temperature mapper measurements aboard the National Science Foundation/National Center for Atmospheric Research Gulfstream V. These measurements are further complemented by limited area simulations using a numerical weather prediction model. This unique data set confirms that strong tropospheric forcing can cause large‐amplitude gravity waves in the mesosphere, and that three essential ingredients are required to achieve this: first, nearly linear propagation across the tropopause; second, leakage through the stratospheric wind minimum; and third, amplification in the polar night jet. Stationary gravity waves were detected in all atmospheric layers up to the mesosphere with horizontal wavelengths between 20 and 100 km. The complete coverage of our data set from troposphere to mesosphere proved to be valuable to identify the processes involved in deep gravity wave propagation.

Abstract. An innovative calibration method for the wind speed measurement using a boom-mounted Rosemount model 858 AJ air velocity probe is introduced. The method is demonstrated for a sensor system installed on a mediumsize research aircraft which is used for measurements in the atmospheric boundary layer. The method encounters a series of coordinated flight manoeuvres to directly estimate the aerodynamic influences on the probe and to calculate the measurement uncertainties. The introduction of a differential Global Positioning System (DGPS) combined with a highaccuracy inertial reference system (IRS) has brought major advances to airborne measurement techniques. The exact determination of geometrical height allows the use of the pressure signal as an independent parameter. Furthermore, the exact height information and the stepwise calibration process lead to maximum accuracy. The results show a measurement uncertainty for the aerodynamic influence of the dynamic and static pressures of 0.1 hPa. The applied parametrisation does not require any height dependencies or time shifts. After extensive flight tests a correction for the flow angles (attack and sideslip angles) was found, which is necessary for a successful wind calculation. A new method is demonstrated to correct for the aerodynamic influence on the sideslip angle. For the three-dimensional (3-D) wind vector (with 100 Hz resolution) a novel error propagation scheme is tested, which determines the measurement uncertainties to be 0.3 m s −1 for the horizontal and 0.2 m s −1 for the vertical wind components.

Abstract. A severe reduction of greenhouse gas emissions is necessary to reach the objectives of the Paris Agreement. The implementation and continuous evaluation of mitigation measures requires regular independent information on emissions of the two main anthropogenic greenhouse gases, carbon dioxide (CO2) and methane (CH4). Our aim is to employ an observation-based method to determine regional-scale greenhouse gas emission estimates with high accuracy. We use aircraft- and ground-based in situ observations of CH4, CO2, carbon monoxide (CO), and wind speed from two research flights over the Upper Silesian Coal Basin (USCB), Poland, in summer 2018. The flights were performed as a part of the Carbon Dioxide and Methane (CoMet) mission above this European CH4 emission hot-spot region. A kriging algorithm interpolates the observed concentrations between the downwind transects of the trace gas plume, and then the mass flux through this plane is calculated. Finally, statistic and systematic uncertainties are calculated from measurement uncertainties and through several sensitivity tests, respectively. For the two selected flights, the in-situ-derived annual CH4 emission estimates are 13.8±4.3 and 15.1±4.0 kg s−1, which are well within the range of emission inventories. The regional emission estimates of CO2, which were determined to be 1.21±0.75 and 1.12±0.38 t s−1, are in the lower range of emission inventories. CO mass balance emissions of 10.1±3.6 and 10.7±4.4 kg s−1 for the USCB are slightly higher than the emission inventory values. The CH4 emission estimate has a relative error of 26 %–31 %, the CO2 estimate of 37 %–62 %, and the CO estimate of 36 %–41 %. These errors mainly result from the uncertainty of atmospheric background mole fractions and the changing planetary boundary layer height during the morning flight. In the case of CO2, biospheric fluxes also add to the uncertainty and hamper the assessment of emission inventories. These emission estimates characterize the USCB and help to verify emission inventories and develop climate mitigation strategies.