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Affect has been identified across numerous research studies to be a vital element in understanding couple relationship processes. Affect has been shown to distinguish between satisfied and dissatisfied couples and to be important in understanding processes leading to relationship dissolution. However, research has not yet uncovered nonverbal indicators that a couple is experiencing negative affect compared to other affective states. In this study we sought to identify specific nonverbal behaviors associated with different affective states. Results suggested that differences in looking-behavior and smiling can be used to identify affect states during couple communication. We outline how the results can aid couples therapy interventions.