The radiation pressure of next generation ultra-high intensity (>10 23 W cm −2 ) lasers could efficiently accelerate ions to GeV energies. However, nonlinear quantum-electrodynamic effects play an important role in the interaction of these laser pulses with matter. Here we show that these effects may lead to the production of an extremely dense (∼10 24 cm −3 ) pair-plasma which absorbs the laser pulse consequently reducing the accelerated ion energy and laser to ion conversion efficiency by up to 30%-50% and 50%-65%, respectively. Thus we identify the regimes of laser-matter interaction, where either ions are efficiently accelerated to high energy or dense pair-plasmas are produced as a guide for future experiments.

Using plasma mirror injection we demonstrate, both analytically and numerically, that a circularly polarized helical laser pulse can accelerate highly collimated dense bunches of electrons to several hundred MeV using currently available laser systems. The circular-polarized helical (Laguerre–Gaussian) beam has a unique field structure where the transverse fields have helix-like wave-fronts which tend to zero on-axis where, at focus, there are large on-axis longitudinal magnetic and electric fields. The acceleration of electrons by this type of laser pulse is analyzed as a function of radial mode number and it is shown that the radial mode number has a profound effect on electron acceleration close to the laser axis. Using three-dimensional particle-in-cell simulations a circular-polarized helical laser beam with power of 0.6 PW is shown to produce several dense attosecond bunches. The bunch nearest the peak of the laser envelope has an energy of 0.47 GeV with spread as narrow as 10%, a charge of 26 pC with duration of ∼ 400 as, and a very low divergence of 20 mrad. The confinement by longitudinal magnetic fields in the near-axis region allows the longitudinal electric fields to accelerate the electrons over a long period after the initial reflection. Both the longitudinal E and B fields are shown to be essential for electron acceleration in this scheme. This opens up new paths toward attosecond electron beams, or attosecond radiation, at many laser facilities around the world.

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We report on the picosecond dynamics of a near-solid-density plasma generated by an intense, infrared (λ = 800 nm) femtosecond laser using time-resolved pump-probe Doppler spectrometry. An initial red-shift is observed in the reflected third harmonic (λ = 266 nm) probe pulse, which gets blue-shifted at longer probe-delays. A combination of particle-in-cell and radiation-hydrodynamics modelling is performed to model the pump laser interaction with the solid target. The results are post-processed to predict the Doppler shift. An excellent agreement is found between the results of such modelling and the experiment. The modelling suggests that the initial inward motion of the critical surface observed in the experiment is due to the passage of a shock-wave-like disturbance, launched by the pump interaction, propagating into the target. Furthermore, in order to achieve the best possible fit to the experimental data, it was necessary to incorporate the effects of bulk ion-acceleration resulting from the electrostatic field set up by the expulsion of electrons from the laser envelope. We also present results of time-resolved pump-probe reflectometry, which are corroborated with the spectrometry results using a 1-D reflectivity model.

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