Atmospheric boundary layer height (ABLH) was observed by the CHM15k ceilometer (January 2008 to October 2013) and the PollyXT lidar (July 2013 to December 2018) over the European Aerosol Research LIdar NETwork to Establish an Aerosol Climatology (EARLINET) site at the Remote Sensing Laboratory (RS-Lab) in Warsaw, Poland. Out of a maximum number of 4017 observational days within this period, a subset of quasi-continuous measurements conducted with these instruments at the same wavelength (1064 nm) was carefully chosen. This provided a data sample of 1841 diurnal cycle ABLH observations. The ABLHs were derived from ceilometer and lidar signals using the wavelet covariance transform method (WCT), gradient method (GDT), and standard deviation method (STD). For comparisons, the rawinsondes of the World Meteorological Organization (WMO 12374 site in Legionowo, 25 km distance to the RS-Lab) were used. The ABLHs derived from rawinsondes by the skew-T-log-p method and the bulk Richardson (bulk-Ri) method had a linear correlation coefficient (R2) of 0.9 and standard deviation (SD) of 0.32 km. A comparison of the ABLHs obtained for different methods and instruments indicated a relatively good agreement. The ABLHs estimated from the rawinsondes with the bulk-Ri method had the highest correlations, R2 of 0.80 and 0.70 with the ABLHs determined using the WCT method on ceilometer and lidar signals, respectively. The three methods applied to the simultaneous, collocated lidar, and ceilometer observations (July to October 2013) showed good agreement, especially for the WCT method (R2 of 0.94, SD of 0.19 km). A scaling threshold-based algorithm was proposed to homogenize ceilometer and lidar datasets, which were applied on the lidar data, and significantly improved the coherence of the results (R2 of 0.98, SD of 0.11 km). The difference of ABLH between clear-sky and cloudy conditions was on average below 230 m for the ceilometer and below 70 m for the lidar retrievals. The statistical analysis of the long-term observations indicated that the monthly mean ABLHs varied throughout the year between 0.6 and 1.8 km. The seasonal mean ABLH was of 1.16 ± 0.16 km in spring, 1.34 ± 0.15 km in summer, 0.99 ± 0.11 km in autumn, and 0.73 ± 0.08 km in winter. In spring and summer, the daytime and nighttime ABLHs appeared mainly in a frequency distribution range of 0.6 to 1.0 km. In winter, the distribution was common between 0.2 and 0.6 km. In autumn, it was relatively balanced between 0.2 and 1.2 km. The annual mean ABLHs maintained between 0.77 and 1.16 km, whereby the mean heights of the well-mixed, residual, and nocturnal layer were 1.14 ± 0.11, 1.27 ± 0.09, and 0.71 ± 0.06 km, respectively (for clear-sky conditions). For the whole observation period, the ABLHs below 1 km constituted more than 60% of the retrievals. A strong seasonal change of the monthly mean ABLH diurnal cycle was evident; a mild weakly defined autumn diurnal cycle, followed by a somewhat flat winter diurnal cycle, then a sharp transition to a spring diurnal cycle, and a high bell-like summer diurnal cycle. A prolonged summertime was manifested by the September cycle being more similar to the summer than autumn cycles.
During August 2016, a quasi-stationary high-pressure system spreading over Central and NorthEastern Europe, caused weather conditions that allowed for 24/7 observations of aerosol optical properties by using a complex multi-wavelength PollyXT lidar system with Raman, polarization and water vapour capabilities, based at the European Aerosol Research Lidar Network (EARLINET network) urban site in Warsaw, Poland. During 24-30 August 2016, the lidar-derived products (boundary layer height, aerosol optical depth, Ångström exponent, lidar ratio, depolarization ratio) were analysed in terms of air mass transport (HYSPLIT model), aerosol load (CAMS data) and type (NAAPS model) and confronted with active and passive remote sensing at the ground level (PolandAOD, AERONET, WIOS-AQ networks) and aboard satellites (SEVIRI, MODIS, CATS sensors). Optical properties for less than a day-old fresh biomass burning aerosol, advected into Warsaw's boundary layer from over Ukraine, were compared with the properties of long-range transported 3-5 day-old aged biomass burning aerosol detected in the free troposphere over Warsaw. Analyses of temporal changes of aerosol properties within the
Abstract. PollyXT Raman polarization lidar observations were performed at the Remote Sensing Laboratory (RS-Lab) in Warsaw (52.2109∘ N, 20.9826∘ E), Poland, in the framework of the European Aerosol Research Lidar Network (EARLINET) and the Aerosol, Clouds, and Trace gases Research Infrastructure (ACTRIS) projects. Data collected in July, August, and September of 2013, 2015, and 2016 were analysed using the classical Raman approach. In total, 246 sets of intact profiles, each set comprising particle extinction (α) and backscatter coefficients (β) as well as linear particle depolarization ratios (δ) at 355 nm and 532 nm, were derived for statistical investigations and stored in the EARLINET/ACTRIS database. The main analysis was focused on intensive optical properties obtained within the atmospheric boundary layer (ABL). Their interrelations were discussed for different periods: the entire day; nighttime, with respect to the nocturnal boundary layer (NL) and the residual boundary layer (RL); at sunrise, with respect to the morning transition boundary layer (MTL); and from late afternoon until sunset, with respect to the well-mixed boundary layer (WML). Within the boundary layer, the lidar-derived optical properties (entire day, 246 sets) revealed a mean aerosol optical depth (AODABL) of 0.20±0.10 at 355 nm and 0.11±0.06 at 532 nm; a mean Ångström exponent (ÅEABL) of 1.54±0.37; a mean lidar ratio (LRABL) of 48±17 sr at 355 nm and 41±15 sr at 532 nm; a mean linear particle depolarization ratio (δABL) of 0.02±0.01 at 355 nm and 0.05±0.01 at 532 nm; and a mean water vapour mixing ratio (WVABL) of 8.28±2.46 g kg−1. In addition, the lidar-derived daytime boundary layer optical properties (for the MTL and WML) were compared with the corresponding daytime columnar aerosol properties derived from the multi-filter rotating shadowband radiometer (MFR-7) measuring within the National Aerosol Research Network (PolandAOD-NET) and the CE318 sun photometer of the Aerosol Robotic NETwork (AERONET). A high linear correlation of the columnar aerosol optical depth values from the two latter instruments was obtained in Warsaw (a correlation coefficient of 0.98 with a standard deviation of 0.02). The contribution of the aerosol load in the summer and early-autumn free troposphere can result in an AODCL value that is twice as high as the AODABL over Warsaw. The occurrence of a turbulence-driven aerosol burst from the boundary layer into the free troposphere can further increase this difference. Aerosol within the ABL and in the free troposphere was interpreted based on comparisons of the properties derived at different altitudes with values reported in the literature, which were characteristic for different aerosol types, in combination with backward trajectory calculations, satellite data, and model outputs. Within the boundary layer, the aerosol consisted of either urban anthropogenic pollution (∼ 61 %) or mixtures of anthropogenic aerosol with biomass-burning aerosol (< 14 %), local pollen (< 7 %), or Arctic marine particles (< 5 %). No significant contribution of mineral dust was found in the boundary layer. The lidar-derived atmospheric boundary layer height (ABLH) and the AODABL exhibited a positive correlation (R of 0.76), associated with the local anthropogenic pollution (most pronounced for the RL and WML). A positive correlation of the AODABL and LRABL and a negative correlation of the ÅEABL and LRABL, as well as the expected negative trends for the WVABL (and surface relative humidity, RH) and δABL, were observed. Relations of the lidar-derived aerosol properties within the ABL and the surface in situ measurements of particulate matter with an aerodynamic diameter less than 10 µm (PM10) and less than 2.5 µm (PM2.5) measured by the Warsaw Regional Inspectorate for Environmental Protection (WIOS) network, and the fine-to-coarse mass ratio (FCMR) were investigated. The FCMR and surface RH showed a positive correlation even at nighttime (R of 0.71 for the MTL, 0.63 for the WML, and 0.6 for the NL), which generally lacked statistically significant relations. A weak negative correlation of the FCMR and δABL (more pronounced at 532 nm at nighttime) and no casual relation between the FCMR and ÅEABL were found. Most interestingly, distinct differences were observed for the morning transition layer (MTL) and the well-mixed layer (WML). The MTL ranged up to 0.6–1 km, and was characterized by a lower AODABL(<0.12), wetter conditions (RH 50–80 %), smaller particles (ÅEABL of 1–2.2; FCMR from 0.5 to 3), and a low LRABL of between 20 and 40 sr. The WML ranged up to 1–2.5 km and exhibited a higher AODABL (reaching up to 0.45), drier conditions (RH 25–60 %), larger particles (ÅEABL of 0.8–1.7; FCMR of 0.2–1.5), and a higher LRABL of up to 90 sr.
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