We find experimentally that the optical sheet conductance of graphite per graphene layer is very close to =2e 2 =h, which is the theoretically expected value of dynamical conductance of isolated monolayer graphene. Our calculations within the Slonczewski-Weiss-McClure model explain well why the interplane hopping leaves the conductance of graphene sheets in graphite almost unchanged for photon energies between 0.1 and 0.6 eV, even though it significantly affects the band structure on the same energy scale. The f-sum rule analysis shows that the large increase of the Drude spectral weight as a function of temperature is at the expense of the removed low-energy optical spectral weight of transitions between hole and electron bands.
We present infrared spectra ͑0.1-1 eV͒ of electrostatically gated bilayer graphene as a function of doping and compare it with tight-binding calculations. All major spectral features corresponding to the expected interband transitions are identified in the spectra: a strong peak due to transitions between parallel split-off bands and two onset-like features due to transitions between valence and conduction bands. A strong gate voltage dependence of these structures and a significant electron-hole asymmetry are observed that we use to extract several band parameters. The structures related to the gate-induced band gap are less pronounced in the experiment than predicted by the tight-binding model that uses parameters obtained from previous experiments on graphite and recent self-consistent band-gap calculations.
Cuprate high-T c superconductors exhibit enigmatic behavior in the nonsuperconducting state. For carrier concentrations near "optimal doping" (with respect to the highest T c s) the transport and spectroscopic properties are unlike those of a Landau-Fermi liquid. On the Mott-insulating side of the optimal carrier concentration, which corresponds to underdoping, a pseudogap removes quasiparticle spectral weight from parts of the Fermi surface and causes a breakup of the Fermi surface into disconnected nodal and antinodal sectors. Here, we show that the near-nodal excitations of underdoped cuprates obey Fermi liquid behavior. The lifetime τ(ω, T) of a quasi-particle depends on its energy ω as well as on the temperature T. For a Fermi liquid, 1/τ(ω, T) is expected to collapse on a universal function proportional to (h ω) 2 + (pπk B T) 2 . Magnetotransport experiments, which probe the properties in the limit ω = 0, have provided indications for the presence of a T 2 dependence of the dc (ω = 0) resistivity of different cuprate materials. However, Fermi liquid behavior is very much about the energy dependence of the lifetime, and this can only be addressed by spectroscopic techniques. Our optical experiments confirm the aforementioned universal ω-and T dependence of 1/τ(ω, T), with p ∼ 1.5. Our data thus provide a piece of evidence in favor of a Fermi liquid-like scenario of the pseudogap phase of the cuprates.optical spectroscopy | superconductivity | mass renormalization | self energy T he compound HgBa 2 CuO 4+δ (Hg1201) is the single-layer cuprate that exhibits the highest T c (97 K). We therefore measured the optical conductivity of strongly underdoped single crystals of Hg1201 ðT c = 67 KÞ. Here we are interested in the optical conductivity of the CuO 2 layers. We therefore express the optical conductivity as a 2D sheet conductance GðωÞ = d c σðωÞ, where d c is the interlayer spacing. The real part of the sheet conductance normalized by the conduction quantum G 0 = 2e 2 =h is shown in Fig. 1. As seen in the figure, a gap-like suppression below 140 meV is clearly observable for temperatures below T c and remains visible in the normal state up to ∼250 K. This is a clear optical signature of the pseudogap. We also observe the zero-energy mode due to the free charge carrier response, which progressively narrows upon lowering the temperature. In materials where the charge carrier relaxation is dominated by impurity scattering, the width of this "Drude" peak corresponds to the relaxation rate of the charge carriers. Relaxation processes arising from interactions have the effect of replacing the constant (frequency-independent) relaxation rate with a frequencydependent one. The general expression for the optical conductivity of interacting electrons is then Gðω; TÞ = iπK Zω + Mðω; TÞ G 0 :[1]The spectral weight K corresponds to minus the kinetic energy if the frequency integration of the experimental data is restricted to intraband transitions. The effect of electron-electron interactions and coupling to collective mo...
We take advantage of the connection between the free-carrier optical conductivity and the glue function in the normal state, to reconstruct from the infrared optical conductivity the glue spectrum of ten different high-T c cuprates revealing a robust peak in the 50-60 meV range and a broad continuum at higher energies for all measured charge-carrier concentrations and temperatures up to 290 K. We observe that the strong-coupling formalism accounts fully for the known strong temperature dependence of the optical spectra of the high-T c cuprates, except for strongly underdoped samples. We observe a correlation between the doping trend of the experimental glue spectra and the critical temperature. The data obtained on the overdoped side of the phase diagram conclusively exclude the electron-phonon coupling as the main source of superconducting pairing.
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