In general circulation models, clouds are parameterized and radiative transfer calculations are performed using the plane-parallel approximation over the cloudy fraction of each model grid. The albedo bias resulting from the plane-parallel representation of spatially heterogeneous clouds has been extensively studied, but the impact of entrainment-mixing processes on cloud microphysics has been neglected up to now. In this paper, this issue is examined by using large-eddy simulations of stratocumulus clouds and tridimensional calculations of radiative transfer in the visible and near-infrared ranges. Two extreme scenarios of mixing are tested: the homogeneous mixing scheme with constant concentration and reduced droplet sizes, against the inhomogeneous mixing scheme, with reduced concentration and constant droplet sizes. The tests reveal that entrainment-mixing effects at cloud top may substantially bias the simulated albedo. In the worse case, which corresponds to a fragmented and thin stratocumulus cloud, the albedo bias changes from Ϫ3% to Ϫ31% when using both mixing schemes alternatively.

Abstract. Detailed ship plume simulations in various convective boundary layer situations have been performed using a Lagrangian Dispersion Model driven by a Large Eddy Simulation Model. The simulations focus on the early stage (1-2 h) of plume dispersion regime and take into account the effects of plume rise on dispersion. Results are presented in an attempt to provide to atmospheric chemistry modellers a realistic description of characteristic dispersion impact on exhaust ship plume chemistry. Plume dispersion simulations are used to derive analytical dilution rate functions. Even though results exhibit striking effects of plume rise parameter on dispersion patterns, it is shown that initial buoyancy fluxes at ship stack have a minor effect on plume dilution rate. After initial high dispersion regimes a simple characteristic dilution time scale can be used to parameterize the subgrid plume dilution effect in large-scale chemistry models. The results show that this parameter is directly related to the typical turn-over time scale of the convective boundary layer.

Two-moment multiclass microphysics schemes are very promising tools to be used in high-resolution NWP models. However, they must be adapted for coarser resolutions. Here, a twofold solution is proposed—namely, a simple representation of subgrid cloud and precipitation fraction—as well as a microphysical sub-time-stepping method. The scheme is easy to implement, allows supersaturation in ice cloud, and exhibits flexibility for adoption across model grid spacing. It is implemented in the Milbrandt and Yau two-moment microphysics scheme with prognostic precipitation in the context of a simple 1D kinematic model as well as a mesoscale NWP model [the Canadian regional Global Environmental Multiscale model (GEM)]. Sensitivity tests were performed and the results highlighting the advantages and disadvantages of the two-moment multiclass cloud scheme relative to the classical Sundqvist scheme. The respective roles of subgrid cloud fraction, precipitation fraction, and time splitting were also studied. When compared to the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO)/CloudSat-retrieved cloud mask, cloud fraction, and ice water content, it is found that the proposed solutions significantly improve the behavior of the Milbrandt and Yau microphysics scheme at the regional NWP scale, suggesting that the subgrid cloud and precipitation fraction technique can be used across model resolutions.

A parameterization for the subgrid-scale cloud and precipitation fractions has been incorporated into the Predicted Particle Properties (P3) microphysics scheme for use in atmospheric models with relatively coarse horizontal resolution. The modified scheme was tested in a simple 1D kinematic model and in the Canadian Global Environmental Multiscale (GEM) model using an operational global NWP configuration with a 25-km grid spacing. A series of 5-day forecast simulations was run using P3 and the much simpler operational Sundqvist condensation scheme as a benchmark for comparison. The effects of using P3 in a global GEM configuration, with and without the modifications, were explored through statistical metrics of common forecast fields against upper-air and surface observations. Diagnostics of state variable tendencies from various physics parameterizations were examined to identify possible sources of errors resulting from the use of the modified scheme. Sensitivity tests were performed on the coupling between the deep convection parameterization scheme and the microphysics, specifically regarding assumptions in the physical properties of detrained ice. It was found that even without re-calibration of the suite of moist physical parameterizations, substituting the Sundqvist condensation scheme with the modified P3 microphysics resulted in some significant improvements to the temperature and geopotential height bias throughout the troposphere and out to day 5, but with degradation to error standard deviation towards the end of the integrations, as well as an increase in the positive bias of precipitation quantities. The modified P3 scheme was thus shown to hold promise for potential use in coarse-resolution NWP systems.