The plane-parallel model for the parameterization of clouds in global climate models is examined in order to estimate the effects of the vertical profile of the microphysical parameters on radiative transfer calculations for extended boundary layer clouds. The vertically uniform model is thus compared to the adiabatic stratified one. The validation of the adiabatic model is based on simultaneous measurements of cloud microphysical parameters in situ and cloud radiative properties from above the cloud layer with a multispectral radiometer. In particular, the observations demonstrate that the dependency of cloud optical thickness on cloud geometrical thickness is larger than predicted with the vertically uniform model and that it is in agreement with the prediction of the adiabatic one. Numerical simulations of the radiative transfer have been performed to establish the equivalence between the two models in terms of the effective radius. They show that the equivalent effective radius of a vertically uniform model is between 80% and 100% of the effective radius at the top of an adiabatic stratified model. The relationship depends, in fact, upon the cloud geometrical thickness and droplet concentration. Remote sensing measurements of cloud radiances in the visible and near infrared are then examined at the scale of a cloud system for a marine case and the most polluted case sampled during the second Aerosol Characterization Experiment. The distributions of the measured values are significantly different between the two cases. This constitutes observational evidence of the aerosol indirect effect at the scale of a cloud system. Finally, the adiabatic stratified model is used to develop a procedure for the retrieval of cloud geometrical thickness and cloud droplet number concentration from the measurements of cloud radiances. It is applied to the marine and to the polluted cases. The retrieved values of droplet concentration are significantly underestimated with respect to the values measured in situ. Despite this discrepancy the procedure is efficient at distinguishing the difference between the two cases.

Thermodynamical and microphysical measurements collected in convective clouds are examined within the frame of the homogeneous/inhomogeneous mixing concept, to determine how entrainment-mixing processes affect cloud droplets, their number concentration, and their mean size. The three selected case studies-one stratocumulus layer and two cumulus clouds-exhibit very different values of the cloud updraft intensity, of the adiabatic droplet mean volume diameter, and of the saturation deficit in the environment, all three parameters that are expected to govern the microphysical response to entrainment mixing. The results confirm that the observed microphysical features are sensitive to the droplet response time to evaporation and to the turbulent homogenization time scale, as suggested by the inhomogeneous mixing concept. They also reveal that an instrumental artifact due to the heterogeneous spatial droplet distribution may be partly responsible for the observed heterogeneous mixing features. The challenge remains, however, to understand why spatially homogeneous cloud volumes larger than the instrument resolution scale (10 m) are so rarely observed. The analysis of the buoyancy of the cloud and clear air mixtures suggests that dynamical sorting could also be efficient for the selection, among all possible mixing scenarios, of those that minimize the local buoyancy production.

In this survey we consider the impact of turbulence on cloud formation from the cloud scale to the droplet scale. We assess progress in understanding the effect of turbulence on the condensational and collisional growth of droplets and the effect of entrainment and mixing on the droplet spectrum. The increasing power of computers and better experimental and observational techniques allow for a much more detailed study of these processes than was hitherto possible. However, much of the research necessarily remains idealized and we argue that it is those studies which include such fundamental characteristics of clouds as droplet sedimentation and latent heating that are most relevant to clouds. Nevertheless, the large body of research over the last decade is beginning to allow tentative conclusions to be made. For example, it is unlikely that small-scale turbulent eddies (i.e. not the energy-containing eddies) alone are responsible for broadening the droplet size spectrum during the initial stage of droplet growth due to condensation. It is likely, though, that small-scale turbulence plays a significant role in the growth of droplets through collisions and coalescence. Moreover, it has been possible through detailed numerical simulations to assess the relative importance of different processes to the turbulent collision kernel and how this varies in the parameter space that is important to clouds. The focus of research on the role of turbulence in condensational and collisional growth has tended to ignore the effect of entrainment and mixing and it is arguable that they play at least as important a role in the evolution of the droplet spectrum. We consider the role of turbulence in the mixing of dry and cloudy air, methods of quantifying this mixing and the effect that it has on the droplet spectrum. Copyright

Abstract. In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan-European aerosol emissions inventory was developed and evaluated, a new cluster spectrometer was built and tested in the field and several new aerosol parameterizations and computations modules for chemical transport and global climate models were developed and evaluated. These achievements and related studies have substantially improved our understanding and reduced the uncertainties of aerosol radiative forcing and air quality-climate interactions. The EUCAARI results can be utilized in European and global environmental policy to assess the aerosol impacts and the corresponding abatement strategies.