Waveform-stabilized laser pulses have revolutionized the exploration of the electronic structure and dynamics of matter by serving as the technological basis for frequency-comb and attosecond spectroscopy. Their primary sources, mode-locked titanium-doped sapphire lasers and erbium/ytterbium-doped fibre lasers, deliver pulses with several nanojoules energy, which is insufficient for many important applications. Here we present the waveform-stabilized light source that is scalable to microjoule energy levels at the full (megahertz) repetition rate of the laser oscillator. A diode-pumped Kerr-lens-mode-locked Yb:YAG thin-disk laser combined with extracavity pulse compression yields waveform-stabilized few-cycle pulses (7.7 fs, 2.2 cycles) with a pulse energy of 0.15 μJ and an average power of 6 W. The demonstrated concept is scalable to pulse energies of several microjoules and near-gigawatt peak powers. The generation of attosecond pulses at the full repetition rate of the oscillator comes into reach. The presented system could serve as a primary source for frequency combs in the mid infrared and vacuum UV with unprecedented high power levels.

We combine high-finesse optical resonators and spatial-spectral interferometry to a highly phase-sensitive investigation technique for nonlinear light-matter interactions. We experimentally validate an ab initio model for the nonlinear response of a resonator housing a gas target, permitting the global optimization of intracavity conversion processes like high-order harmonic generation. We predict the feasibility of driving intracavity high-order harmonic generation far beyond intensity limitations observed in state-of-the-art systems by exploiting the intracavity nonlinearity to compress the pulses in time.

The feed-forward technique has recently revolutionized carrier-envelope phase (CEP) stabilization, enabling unprecedented values of residual phase jitter. Nevertheless, its demonstrations have hitherto remained in a proof-of-principle state. Here we show that pulse quality and power issues can be solved, leading to few-cycle pulses with good beam quality. Making use of stable interferometers, we achieve day-long CEP-stable operation of the setup. Out-of-loop RMS phase noise amounts to less than 30 mrad in 20 s, with more than 24 h of CEP-locked operation being demonstrated.

The demand for ever shorter light pulses presents a challenge to the detection and stabilization of the carrier-envelope phase (CEP) in amplifier systems. Here we present a combination of single-shot detection and a fast actuator that is capable of measuring and correcting the CEP in every single shot emitted by a millijoule-scale, multi-kHz femtosecond laser amplifier. The residual CEP noise within 50 s amounts to 98 mrad rms in-loop (fast detection, 5·10⁵ shots) and 140 mrad out-of-loop (slow detection, 6250 shots), approaching the noise floor of the f-to-2f measurement. Both values represent a twofold improvement of the CEP stability over previously published results in comparable systems.

The optimal enhancement of broadband optical pulses in a passive resonator requires a seeding pulse train with a specific carrier-envelope-offset frequency. Here, we control the phase of the cavity mirrors to tune the offset frequency for which a given comb is optimally enhanced. This enables the enhancement of a zero-offset-frequency train of sub-30-fs pulses to multi-kW average powers. The combination of pulse duration, power, and zero phase slip constitutes a crucial step toward the generation of attosecond pulses at multi-10-MHz repetition rates. In addition, this control affords the enhancement of pulses generated by difference-frequency mixing, e.g., for mid-infrared spectroscopy.