Self-assembled binary multichromophore dendrimers HDSD–FDSD have been developed to increase the poling efficiency, refractive Index and stability of the EO materials.

Four nonlinear optical chromophores A–D functionalized with different isolation groups on both the donor and bridge sections of the chromophores have been synthesized and systematically investigated.

A series of nonlinear optical chromophores A–D based on the diethylaminophenyl donor and tricyanofuran or phenyl-trifluoromethyl-tricyanofuran acceptors coupled through a tetraene bridge was synthesized and investigated.

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