Rontgenstrukturanalyse sowie die eindeutigen Deuterierungsergebnisse sprechen fur einen stereochemisch einheitlichen Verlauf der Umlagerungen. Sterische und elektronische Einflusse auf einige analoge Umlagerungen werden untersucht, der Mechanisnus wird diskutiert.Thermal Rearrangements of 1-Allyloxy-and I-Propargyloxy-A5-phosphorin Derivatives The thermal rearrangements of l-allyloxy-h'-phosphorin derivatives 1 affords -contrary to the formally similar Claisen rearrangement of ally1 phenyl ethers -in the irreversible step an ,,antiWoodward-Hoffmann" [3,5,] ally1 shift to 4-allyl-1 ,Cdihydro-h'-phosphorin derivatives 2. -The reaction is, as cross experiments prove, intramolecular and stereospecific according to 1' ' order law. It is accelerated by electron donating substituents in position 4 and by electron attracting substituents at the phosphorus, but is not much solvent-dependant. In a next step, again with allyl-inversion, a [3,3,] Cope rearrangement follows to give 2-allyl-1 ,2-dihydro-h5-phosphorin derivatives 3. At somewhat higher temperature, by an intramolecular [4 + 21-cycloaddition from 3 a tricyclus 4 is formed. Besides the experiments with deuterium marked compounds, the X-ray analysis of 4 proves the uniform stereochemic way of all these rearrangements. Steric and electronic influences on some analogous rearrangements are studied, the mechanism is discussed.I-Allyloxy-1'-phosphorin-Derivate der allgemeinen Konstitution 1 lagern sich beim Erhitzen in indifferenten Losungsmitteln unter Wanderung der Allylgruppe vom Sauerstoff an das Ringkohlenstoffatom 42) in formal ahnlicher Weise wie Allylphenylether bei der Clai~en-Umlagerung~) urn. Der wesentliche Unterschied besteht darin, daB im Primarschritt nicht das 2-sondern das CAllyl-Derivat gebildet wird, wobei zugleich, wie Deuterierungsversuche beweisen, Allylumkehr (la' -+ 2a') eintritt.Die Umlagerung erfolgt somit in einer den Woodward-Hoffmann-Regeln scheinbar widersprechenden [3,5,]-sigmatropen Wanderung. Die Reaktion lafit sich sehr bequem 'H-NMR-spektroskopisch verfolgen und ist irn Gegensatz zu einer friiher beobachteten
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